Non-Fully Conjugated Dimerized Giant Acceptors with Different Alkyl-Linked Sites for Stable and 19.13 % Efficiency Organic Solar Cells
Fan Yi
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorCorresponding Author
Manjun Xiao
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
Search for more papers by this authorYongdie Meng
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
Search for more papers by this authorHairui Bai
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorWenyan Su
School of Materials Science and Engineering, Xi'an University of Science and Technology, Xi'an, 710054 China
Search for more papers by this authorWei Gao
Xiamen Key Laboratory of Optoelectronic Materials and Advanced Manufacturing, Institute of Luminescent Materials and Information Displays, College of Materials Science and Engineering, Huaqiao University, Xiamen, 361021 China
Search for more papers by this authorZe-Fan Yao
College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871 China
Search for more papers by this authorGuangyu Qi
Search for more papers by this authorZezhou Liang
Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi, Key Lab of Photonic Technique for Information, School of Electronics Science & Engineering, Faculty of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorConggui Jin
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
Search for more papers by this authorLingxiao Tang
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorRui Zhang
Department of Physics, Chemistry and Biology (IFM), Linköping University, Linköping, SE-58183 Sweden
Search for more papers by this authorLihe Yan
Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi, Key Lab of Photonic Technique for Information, School of Electronics Science & Engineering, Faculty of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorYuhang Liu
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorWeiguo Zhu
Jiangsu Engineering Laboratory of Light-Electricity-Heat Energy-Converting Materials and Applications, School of Materials Science and Engineering, Changzhou University, Changzhou, 213164 China
Search for more papers by this authorCorresponding Author
Wei Ma
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorCorresponding Author
Qunping Fan
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorFan Yi
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorCorresponding Author
Manjun Xiao
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
Search for more papers by this authorYongdie Meng
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
Search for more papers by this authorHairui Bai
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorWenyan Su
School of Materials Science and Engineering, Xi'an University of Science and Technology, Xi'an, 710054 China
Search for more papers by this authorWei Gao
Xiamen Key Laboratory of Optoelectronic Materials and Advanced Manufacturing, Institute of Luminescent Materials and Information Displays, College of Materials Science and Engineering, Huaqiao University, Xiamen, 361021 China
Search for more papers by this authorZe-Fan Yao
College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871 China
Search for more papers by this authorGuangyu Qi
Search for more papers by this authorZezhou Liang
Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi, Key Lab of Photonic Technique for Information, School of Electronics Science & Engineering, Faculty of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorConggui Jin
College of Chemistry, Key Lab of Environment-Friendly Chemistry and Application (Ministry of Education), Xiangtan University, Xiangtan, 411105
Search for more papers by this authorLingxiao Tang
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorRui Zhang
Department of Physics, Chemistry and Biology (IFM), Linköping University, Linköping, SE-58183 Sweden
Search for more papers by this authorLihe Yan
Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi, Key Lab of Photonic Technique for Information, School of Electronics Science & Engineering, Faculty of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorYuhang Liu
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorWeiguo Zhu
Jiangsu Engineering Laboratory of Light-Electricity-Heat Energy-Converting Materials and Applications, School of Materials Science and Engineering, Changzhou University, Changzhou, 213164 China
Search for more papers by this authorCorresponding Author
Wei Ma
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorCorresponding Author
Qunping Fan
State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, 710049 China
Search for more papers by this authorGraphical Abstract
Three new non-fully conjugated dimerized giant acceptors with different alkyl-linked sites are developed. Among them, wing-sited 2Y-wing has fine-tuned packing and better miscibility with donor, allowing to 19.13 % efficiency (which is the highest value among the devices with giant acceptors) and highly stable organic solar cells.
Abstract
Achieving both high power conversion efficiency (PCE) and device stability is a major challenge for the practical development of organic solar cells (OSCs). Herein, three non-fully conjugated dimerized giant acceptors (named 2Y-sites, including wing-site-linked 2Y-wing, core-site-linked 2Y-core, and end-site-linked 2Y-end) are developed. They share the similar monomer precursors but have different alkyl-linked sites, offering the fine-tuned molecular absorption, packing, glass transition temperature, and carrier mobility. Among their binary active layers, D18/2Y-wing has better miscibility, leading to optimized morphology and more efficient charge transfer compared to D18/2Y-core and D18/2Y-end. Therefore, the D18/2Y-wing-based OSCs achieve a superior PCE of 17.73 %, attributed to enhanced photocurrent and fill factor. Furthermore, the D18/2Y-wing-based OSCs exhibit a balance of high PCE and improved stability, distinguishing them within the 2Y-sites. Building on the success of 2Y-wing in binary systems, we extend its application to ternary OSCs by pairing it with the near-infrared absorbing D18/BS3TSe-4F host. Thanks to the complementary absorption within 300–970 nm and further optimized morphology, ternary OSCs obtain a higher PCE of 19.13 %, setting a new efficiency benchmark for the dimer-derived OSCs. This approach of alkyl-linked site engineering for constructing dimerized giant acceptors presents a promising pathway to improve both PCE and stability of OSCs.
Conflict of interests
The authors declare no conflict of interest.
Open Research
Data Availability Statement
The data that support the findings of this study are available from the corresponding author upon reasonable request.
Supporting Information
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