Preparation of Bi2O3@PCPA-KH590/chloroprene composites with good mechanical properties under high-filling
Jun Zeng
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Writing - original draft (lead)
Search for more papers by this authorCorresponding Author
YingJun Li
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Correspondence
YingJun Li and YuanLin Zhou, School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621900, China.
Email: [email protected] and [email protected]
Contribution: Writing - review & editing (equal)
Search for more papers by this authorYingChun Lu
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorYunPeng Li
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorHuiPing Liu
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Data curation (equal)
Search for more papers by this authorCongXiu Wu
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorMengXi Chen
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorWei OuYang
Zhuzhou Rubber Research & Design Institute Co., Ltd. of Chemchina, China National Chemical Corporation, Zhuzhou, China
Hunan Key Laboratory of Near-Space Meteo-Ballon Materials and Technology, Hunan Provincial Department of Science and Technology, Zhuzhou, China
Contribution: Formal analysis (equal)
Search for more papers by this authorYiPeng Zhang
Zhuzhou Rubber Research & Design Institute Co., Ltd. of Chemchina, China National Chemical Corporation, Zhuzhou, China
Hunan Key Laboratory of Near-Space Meteo-Ballon Materials and Technology, Hunan Provincial Department of Science and Technology, Zhuzhou, China
Contribution: Formal analysis (equal)
Search for more papers by this authorCorresponding Author
YuanLin Zhou
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Correspondence
YingJun Li and YuanLin Zhou, School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621900, China.
Email: [email protected] and [email protected]
Contribution: Writing - review & editing (equal)
Search for more papers by this authorJun Zeng
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Writing - original draft (lead)
Search for more papers by this authorCorresponding Author
YingJun Li
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Correspondence
YingJun Li and YuanLin Zhou, School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621900, China.
Email: [email protected] and [email protected]
Contribution: Writing - review & editing (equal)
Search for more papers by this authorYingChun Lu
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorYunPeng Li
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorHuiPing Liu
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Data curation (equal)
Search for more papers by this authorCongXiu Wu
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorMengXi Chen
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Contribution: Investigation (equal)
Search for more papers by this authorWei OuYang
Zhuzhou Rubber Research & Design Institute Co., Ltd. of Chemchina, China National Chemical Corporation, Zhuzhou, China
Hunan Key Laboratory of Near-Space Meteo-Ballon Materials and Technology, Hunan Provincial Department of Science and Technology, Zhuzhou, China
Contribution: Formal analysis (equal)
Search for more papers by this authorYiPeng Zhang
Zhuzhou Rubber Research & Design Institute Co., Ltd. of Chemchina, China National Chemical Corporation, Zhuzhou, China
Hunan Key Laboratory of Near-Space Meteo-Ballon Materials and Technology, Hunan Provincial Department of Science and Technology, Zhuzhou, China
Contribution: Formal analysis (equal)
Search for more papers by this authorCorresponding Author
YuanLin Zhou
State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang, China
School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang, China
Correspondence
YingJun Li and YuanLin Zhou, School of Materials and Chemistry, Southwest University of Science and Technology, Mianyang 621900, China.
Email: [email protected] and [email protected]
Contribution: Writing - review & editing (equal)
Search for more papers by this authorAbstract
As a “green” radiation protection material with the potential to replace lead oxide, bismuth oxide has more research applications in the field of γ protection. However, due to their different surface properties, there are compatibility and interaction problems between metal oxides and rubber. To enhance the performance of bismuth oxide in neoprene, Bi2O3@PCPA-KH590 was prepared by coating bismuth oxide with polyphenol/polyamine and grafting KH590 on the surface of bismuth oxide. This allows for creating more active sites with the help of polyphenol/polyamine, enabling KH590 to be grafted onto bismuth oxide particles. The S functional group on the silane coupling agent is then cross-linked with the rubber substrate, enhancing the dispersibility of the bismuth oxide powder. This improvement not only improves the dispersibility of the bismuth oxide powder but also enhances the mechanical properties of the rubber composite material. Compared with pure CR, the mechanical properties of 60 wt% filler-modified powder composites can still be maintained at a high level, with the tensile strength reaching 12.83 Mpa. In sum, the proposed method appears feasible for preparing highly filled radiation protection rubber-based materials.
CONFLICT OF INTEREST STATEMENT
The authors declare no conflict of interest.
Open Research
DATA AVAILABILITY STATEMENT
The data that support the findings of this study are available from the corresponding author upon reasonable request.
Supporting Information
| Filename | Description |
|---|---|
| app54782-sup-0001-supinfo.docxWord 2007 document , 1.6 MB | Data S1: Supporting Information. |
Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.
REFERENCES
- 1T. Bachtiar, I. Anas, A. Sutandi, Ishak, IOP Conf. Ser.: Earth Environ. Sci 2022, 951, 012046.
10.1088/1755-1315/951/1/012046 Google Scholar
- 2A. A. Oglat, J. Radiat. Res. Appl. Sci. 2023, 16, 100503.
- 3M. Ahmed, A. S. D. El-Khatib, M. S. Badawi, A. E. Abu-Rayan, N. S. Aly, J. S. Alzahrani, M. I. Abbas, Mater. Res. Express 2020, 7, 105309.
10.1088/2053-1591/abbf9f Google Scholar
- 4M. E. Mahmoud, A. M. El-Khatib, M. S. Badawi, A. R. Rashed, R. M. El-Sharkawy, A. A. Thabet, Radiat. Phys. Chem. 2018, 145, 160.
- 5C. Harrison, S. Weaver, C. Bertelsen, E. Burgett, N. Hertel, E. Grulke, J. Appl. Polym. Sci. 2008, 109, 2529.
- 6J. Kim, D. Seo, B. C. Lee, Y. S. Seo, W. H. Miller, Adv. Eng. Mater. 2014, 16, 1083.
- 7S.-C. Kim, Materials 2022, 15, 1338.
- 8S. Intom, E. Kalkornsurapranee, J. Johns, S. Kaewjaeng, S. Kothan, W. Hongtong, W. Chaiphaksa, J. Kaewkhao, Radiat. Phys. Chem. 2020, 172, 108772.
- 9E. Kalkornsurapranee, S. Kothan, S. Intom, J. Johns, S. Kaewjaeng, C. Kedkaew, W. Chaiphaksa, T. Sareein, J. Kaewkhao, Radiat. Phys. Chem. 2021, 179, 109261.
- 10A. Tohsan, S. Joomcom, W. Limphirat, Mater. Today: Proc. 2018, 5, 9584.
- 11A. Thumwong, E. Wimolmala, T. Markpin, N. Sombatsompop, K. Saenboonruang, Radiat. Phys. Chem. 2021, 186, 109530.
- 12T. Özdemir, A. Güngör, I. K. Akbay, H. Uzun, Y. Babucçuoglu, Radiat. Phys. Chem. 2018, 144, 248.
- 13M. E. Mahmoud, A. M. El-Khatib, M. S. Badawi, A. R. Rashad, R. M. El-Sharkawy, A. A. Thabet, J. Clean. Prod. 2018, 176, 276.
- 14M. Elsafi, M. I. Hanan Al-Ghamdi, A. A. Sayyed, A. H. Almuqrin, K. A. Mahmoud, K. Cornish, T. I. Shalaby, A. M. El-Khatib, J. Mater. Res. Technol. 2022, 19, 1862.
- 15M. M. Abdel-Aziz, S. E. Gwaily, Polym. Degrad. Stab. 1997, 3, 269.
10.1016/S0141-3910(96)00119-X Google Scholar
- 16D. J. Simpkin, Health Phys. 1987, 52, 431.
- 17X. Liu, Q.-P. Zhang, J.-L. Li, R.-C. Chen, W.-D. Xu, Y.-T. Li, W.-B. Yang, Y.-L. Zhou, J. Appl. Polym. Sci. 2022, 139, 51914.
- 18V. N. Gulbin, V. F. Petrunin, Phys. Procedia 2015, 72, 540.
- 19H. Aboud, M. J. R. Aldhuhaibat, Y. Alajermi, Radiat. Phys. Chem. 2022, 191, 109836.
- 20A. El-Sayed Abdoa, M. A. M. Ali, M. R. Ismail, Radiat. Phys. Chem. 2003, 66, 185.
- 21S. Vignesh, J. T. Winowlin Jappes, S. Nagaveena, R. Krishna Sharma, M. Adam Khan, C. V. More, Vacuum 2023, 207, 111583.
- 22I. Kashif, A. Abd El-Maboud, R. El-said, E. M. Sakr, A. A. Soliman, J. Alloys Compd. 2012, 539, 124.
- 23K. Bagheri, S. M. Razavi, S. J. Ahmadi, M. Kosari, H. Abolghasemi, Radiat. Phys. Chem. 2018, 146, 5.
- 24D. A. Aloraini, M. I. Sayyed, K. A. Mahmoud, A. A. H. Almuqrin, A. Kumar, M. U. Khandaker, M. Elsafi, Radiat. Phys. Chem. 2022, 200, 110172.
- 25W. Poltabtim, E. Wimolmala, K. Saenboonruang, Radiat. Phys. Chem. 2018, 153, 1.
- 26S. N. Yılmaz, İ. K. Akbay, T. Özdemir, Radiat. Phys. Chem. 2021, 180, 109316.
- 27Q. Li, R. Zhong, X. Xiao, J.-L. Liao, X.-P. Liao, B. Shi, ACS Appl. Mater. Interfaces 2020, 12, 54117.
- 28S. Park, H. Kim, Y. Kim, E. Kim, Y. Seo, MRS Adv. 2018, 3, 1789.
- 29H. Wang, J.-J. Wu, C. Cai, J. Guo, H.-S. Fan, C.-Z. Zhu, H.-X. Dong, N. Zhao, J. Xu, ACS Appl. Mater. Interfaces 2014, 6, 5602.
- 30D. Yang, L.-Y. Yu, J. Ai, Q.-G. Wei, Y.-F. Ni, L.-Q. Zhang, Compos Commun 2021, 23, 100565.
- 31L. Wang, Y.-X. Shi, S.-X. Chen, W.-C. Wang, M. Tian, N.-Y. Ning, L.-Q. Zhang, Chem. Eng. J. 2016, 314, 583.
- 32D. Yang, Y.-F. Ni, Y.-J. Xu, X.-X. Kong, Y.-C. Feng, L.-Q. Zhang, Polymer 2019, 183, 121813.
- 33D. Yang, Y.-F. Ni, X.-X. Kong, H. Xue, W.-L. Guo, L.-Q. Zhang, Appl. Surf. Sci. 2019, 495, 143638.
- 34W. Tang, C. Chen, W. Sun, P. Wang, D.-Z. Wei, Int. J. Biol. Macromol. 2019, 128, 814.
- 35Q. Wei, D. Yang, L.-Y. Yu, Y.-F. Ni, L.-Q. Zhang, Compos. Sci. Technol. 2020, 199, 108344.
- 36X. Xie, D. Yang, Appl. Surf. Sci. 2022, 602, 154335.
- 37X.-J. Shang, Y.-M. Zhu, Z.-H. Li, Appl. Surf. Sci. 2017, 394, 169.
- 38Z.-P. Wang, H. Zhang, Q. Liu, S.-J. Wang, S.-K. Yan, Mareials 2022, 15, 10.
- 39Y.-X. Liu, J.-X. Liu, Mater. Res. Express. 2018, 6, 035204.
- 40W.-L. Wu, B.-W. Yu, J Rubber Res 2020, 23, 163.
- 41G.-D. Zeng, Y. Zhou, T.-Z. Wang, K. Li, Y.-M. Dong, J.-J. Li, J.-Z. Li, Z. Fang, Chem. Eng. J. 2023, 453, 139761.
- 42M.-Y. Wang, L.-C. Ma, L.-L. Shi, P.-F. Feng, X.-J. Wang, Y.-Y. Zhu, G.-S. Wu, G.-J. Song, Compos. Sci. Technol. 2019, 182, 107751.
- 43D. An, X.-Y. Duan, S.-S. Cheng, Z.-Y. Zhang, B. Yang, Q.-S. Lian, J.-X. Li, Z.-J. Sun, Y.-Q. Liu, C.-P. Wong, Compos Part A-Appl S. 2020, 135, 105928.
- 44Y.-D. Liu, Y.-K. Yuan, J.-H. Liu, J. Hua, Polym. Test. 2021, 101, 107312.
- 45X.-Y. Duan, R.-Z. He, D. An, J. He, R.-Y. Tao, Y.-W. Cui, C.-B. Liang, Z.-J. Sun, Y.-Q. Liu, C.-P. Wong, Diam. Relat. Mater. 2022, 130, 109512.
- 46K.-Q. Luo, W. Zheng, X.-Y. Zhao, X.-J. Wang, S.-Z. Wu, Mater. Des. 2018, 154, 312.
- 47H. Zhang, Y.-J. Li, J. Zeng, H.-P. Liu, Y.-L. Zhou, J. Appl. Polym. Sci. 2022, 139, 52335.
- 48S. Thongsang, N. Sombatsompop, Polym. Compos. 2006, 27, 30.
Citing Literature
