Minireview
Metal–Organic Frameworks Based Electrocatalysts for the Oxygen Reduction Reaction
Dr. Xue Feng Lu,
Prof. Bao Yu Xia,
Prof. Shuang-Quan Zang,
Prof. Xiong Wen (David) Lou,
Dr. Xue Feng Lu
School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore, 637459 Singapore
Search for more papers by this authorProf. Bao Yu Xia
School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology (HUST), 1037 Luoyu Road, Wuhan, 430074 P. R. China
Search for more papers by this authorProf. Shuang-Quan Zang
College of Chemistry and Molecular Engineering, Zhengzhou University, Henan, 450001 P. R. China
Search for more papers by this authorCorresponding Author
Prof. Xiong Wen (David) Lou
School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore, 637459 Singapore
Search for more papers by this authorDr. Xue Feng Lu,
Prof. Bao Yu Xia,
Prof. Shuang-Quan Zang,
Prof. Xiong Wen (David) Lou,
Dr. Xue Feng Lu
School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore, 637459 Singapore
Search for more papers by this authorProf. Bao Yu Xia
School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology (HUST), 1037 Luoyu Road, Wuhan, 430074 P. R. China
Search for more papers by this authorProf. Shuang-Quan Zang
College of Chemistry and Molecular Engineering, Zhengzhou University, Henan, 450001 P. R. China
Search for more papers by this authorCorresponding Author
Prof. Xiong Wen (David) Lou
School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, Singapore, 637459 Singapore
Search for more papers by this authorGraphical Abstract
Despite the rapid developments in the past decade, many great challenges remain for the practical use of metal–organic frameworks (MOFs) based electrocatalysts. This Minireview summaries some major recent research efforts and advances on MOF-based electrocatalysts for the oxygen reduction reaction. Some promising directions and strategies are also discussed.
Abstract
In view of the clean and sustainable energy, metal–organic frameworks (MOFs) based materials, including pristine MOFs, MOF composites, and their derivatives are emerging as unique electrocatalysts for oxygen reduction reaction (ORR). Thanks to their tunable compositions and diverse structures, efficient MOF-based materials provide new opportunities to accelerate the sluggish ORR at the cathode in fuel cells and metal–air batteries. This Minireview first provides some introduction of ORR and MOFs, followed by the classification of MOF-based electrocatalysts towards ORR. Recent breakthroughs in engineering MOF-based ORR electrocatalysts are highlighted with an emphasis on synthesis strategy, component, morphology, structure, electrocatalytic performance, and reaction mechanism. Finally, some current challenges and future perspectives for MOF-based ORR electrocatalysts are also discussed.
Conflict of interest
The authors declare no conflict of interest.
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Citing Literature
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