Site-Specific Synthesis and In Situ Immobilization of Fluorescent Silver Nanoclusters on DNA Nanoscaffolds by Use of the Tollens Reaction†
Suchetan Pal
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
These authors contributed equally.
Search for more papers by this authorDr. Reji Varghese
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
These authors contributed equally.
Search for more papers by this authorDr. Zhengtao Deng
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Search for more papers by this authorZhao Zhao
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Search for more papers by this authorAshok Kumar
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Search for more papers by this authorCorresponding Author
Prof. Hao Yan
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378Search for more papers by this authorCorresponding Author
Prof. Yan Liu
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378Search for more papers by this authorSuchetan Pal
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
These authors contributed equally.
Search for more papers by this authorDr. Reji Varghese
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
These authors contributed equally.
Search for more papers by this authorDr. Zhengtao Deng
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Search for more papers by this authorZhao Zhao
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Search for more papers by this authorAshok Kumar
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Search for more papers by this authorCorresponding Author
Prof. Hao Yan
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378Search for more papers by this authorCorresponding Author
Prof. Yan Liu
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378
Department of Chemistry and Biochemistry and The Biodesign Institute, Arizona State University, Tempe, AZ 85287 (USA), Fax: (+1) 480-727-2378Search for more papers by this authorThis research was partly supported by grants from the ONR, ARO, NSF, DOE, and NIH to Y.L. and from the ONR, ARO, NSF, DOE, NIH, and Sloan Research Foundation to H.Y. Y.L. and H.Y. were supported as part of the Center for Bio-Inspired Solar Fuel Production, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy.
Graphical Abstract
Versilbertes Origami: Durch den Einsatz von DNA-Strängen mit bestimmten Sequenzen können kovalent angebundene Zuckereinheiten gezielt in DNA-Origami-Strukturen eingebaut werden. Dieser Ansatz ermöglicht eine anschließende Synthese und In-situ-Immobilisierung von fluoreszierenden Ag-Nanoclustern an vorgegebenen Positionen des DNA-Gerüsts durch Behandlung mit dem Tollens-Reagens (siehe Bild).
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