Review
Advanced Nanocarbons Toward two-Electron Oxygen Electrode Reactions for H2O2 Production and Integrated Energy Conversion
Linjie Zhao,
Riqing Yan,
Baoguang Mao,
Rajib Paul,
Wenjie Duan,
Liming Dai,
Chuangang Hu,
Linjie Zhao
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorRiqing Yan
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorBaoguang Mao
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorRajib Paul
Advanced Materials and Liquid Crystal Institute, Kent State University, Kent, OH, 44242 USA
Search for more papers by this authorWenjie Duan
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorLiming Dai
Australian Carbon Materials Centre (A-CMC), School of Chemical Engineering, University of New South Wales, Sydney, NSW, 2052 Australia
Search for more papers by this authorCorresponding Author
Chuangang Hu
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
E-mail: [email protected]
Search for more papers by this authorLinjie Zhao,
Riqing Yan,
Baoguang Mao,
Rajib Paul,
Wenjie Duan,
Liming Dai,
Chuangang Hu,
Linjie Zhao
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorRiqing Yan
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorBaoguang Mao
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorRajib Paul
Advanced Materials and Liquid Crystal Institute, Kent State University, Kent, OH, 44242 USA
Search for more papers by this authorWenjie Duan
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
Search for more papers by this authorLiming Dai
Australian Carbon Materials Centre (A-CMC), School of Chemical Engineering, University of New South Wales, Sydney, NSW, 2052 Australia
Search for more papers by this authorCorresponding Author
Chuangang Hu
State Key Laboratory of Organic–Inorganic Composites, Beijing Key Laboratory of Energy Environmental Catalysis, College of Chemical Engineering, Beijing University of Chemical Technology, Beijing, 100029 China
E-mail: [email protected]
Search for more papers by this authorAbstract
Hydrogen peroxide (H2O2) plays a pivotal role in advancing sustainable technologies due to its eco-friendly oxidizing capability. The electrochemical two-electron (2e−) oxygen reduction reaction and water oxidation reaction present an environmentally green method for H2O2 production. Over the past three years, significant progress is made in the field of carbon-based metal-free electrochemical catalysts (C-MFECs) for low-cost and efficient production of H2O2 (H2O2EP). This article offers a focused and comprehensive review of designing C-MFECs for H2O2EP, exploring the construction of dual-doping configurations, heteroatom-defect coupling sites, and strategic dopant positioning to enhance H2O2EP efficiency; innovative structural tuning that improves interfacial reactant concentration and promote the timely release of H2O2; modulation of electrolyte and electrode interfaces to support the 2e− pathways; and the application of C-MFECs in reactors and integrated energy systems. Finally, the current challenges and future directions in this burgeoning field are discussed.
Conflict of Interest
The authors declare no conflict of interest.
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