Low-Frequency Sub-Terahertz Absorption in HgII−XCN−FeII (X=S, Se) Coordination Polymers
Guanping Li
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Data curation (equal), Formal analysis (equal), Investigation (lead), Project administration (equal), Validation (equal), Visualization (lead), Writing - original draft (lead)
Search for more papers by this authorCorresponding Author
Dr. Olaf Stefanczyk
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Conceptualization (equal), Data curation (equal), Formal analysis (supporting), Funding acquisition (supporting), Investigation (supporting), Project administration (equal), Resources (supporting), Supervision (supporting), Validation (equal), Visualization (supporting), Writing - review & editing (equal)
Search for more papers by this authorDr. Kunal Kumar
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Formal analysis (equal), Funding acquisition (supporting), Investigation (supporting), Project administration (supporting), Validation (supporting), Visualization (supporting), Writing - review & editing (supporting)
Search for more papers by this authorYuuki Mineo
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Formal analysis (supporting), Investigation (supporting), Visualization (supporting), Writing - review & editing (supporting)
Search for more papers by this authorDr. Koji Nakabayashi
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Funding acquisition (supporting), Investigation (supporting), Supervision (supporting), Writing - review & editing (supporting)
Search for more papers by this authorCorresponding Author
Prof. Dr. Shin-ichi Ohkoshi
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Conceptualization (equal), Data curation (equal), Funding acquisition (lead), Investigation (supporting), Project administration (equal), Resources (lead), Supervision (lead), Visualization (supporting), Writing - review & editing (equal)
Search for more papers by this authorGuanping Li
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Data curation (equal), Formal analysis (equal), Investigation (lead), Project administration (equal), Validation (equal), Visualization (lead), Writing - original draft (lead)
Search for more papers by this authorCorresponding Author
Dr. Olaf Stefanczyk
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Conceptualization (equal), Data curation (equal), Formal analysis (supporting), Funding acquisition (supporting), Investigation (supporting), Project administration (equal), Resources (supporting), Supervision (supporting), Validation (equal), Visualization (supporting), Writing - review & editing (equal)
Search for more papers by this authorDr. Kunal Kumar
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Formal analysis (equal), Funding acquisition (supporting), Investigation (supporting), Project administration (supporting), Validation (supporting), Visualization (supporting), Writing - review & editing (supporting)
Search for more papers by this authorYuuki Mineo
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Formal analysis (supporting), Investigation (supporting), Visualization (supporting), Writing - review & editing (supporting)
Search for more papers by this authorDr. Koji Nakabayashi
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Funding acquisition (supporting), Investigation (supporting), Supervision (supporting), Writing - review & editing (supporting)
Search for more papers by this authorCorresponding Author
Prof. Dr. Shin-ichi Ohkoshi
Department of Chemistry, School of Science, The University of Tokyo, 7-3-1, Hongo, Bunkyo-ku, Tokyo, 113-0033 Japan
Contribution: Conceptualization (equal), Data curation (equal), Funding acquisition (lead), Investigation (supporting), Project administration (equal), Resources (lead), Supervision (lead), Visualization (supporting), Writing - review & editing (equal)
Search for more papers by this authorAbstract
Self-assembly FeII complexes of phenazine (Phen), quinoxaline (Qxn), and 4,4′-trimethylenedipyridine (Tmp) with tetrahedral building blocks of [HgII(XCN)4]2− (X=S or Se) formed six new high-dimensional frameworks with the general formula of [Fe(L)m][Hg(XCN)4]⋅solvents (L=Phen, m/X=2/S, 1; L=Qxn, m/X=2/S, 2; L=Qxn, m/X=1/S, 3; L=Qxn, m/X=1/Se, 3-Se; L=Tmp, m/X=1/S, 4; and L=Tmp, m/X=1/Se, 4-Se). 1, 3, and 3-Se show an intense sub-terahertz (sub-THz) absorbance of around 0.60 THz due to vibrations of the solvent molecules coordinated to the FeII ions and crystallization organic molecules. In addition, crystals of 1, 4, and 4-Se display low-frequency Raman scattering with exceptionally low values of 0.44, 0.51, and 0.53 THz, respectively. These results indicate that heavy metal FeII−HgII systems are promising platforms to construct sub-THz absorbers.
Conflict of interest
The authors declare no conflict of interest
Open Research
Data Availability Statement
The data that support the findings of this study are available from the corresponding author upon reasonable request.
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