A Highly Ordered Quantum Dot Supramolecular Assembly Exhibiting Photoinduced Emission Enhancement
Corresponding Author
Dr. Mitsuaki Yamauchi
Department of Applied Chemistry for Environment, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337 Japan
Search for more papers by this authorSeiya Yamamoto
Department of Applied Chemistry for Environment, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337 Japan
Search for more papers by this authorCorresponding Author
Prof. Dr. Sadahiro Masuo
Department of Applied Chemistry for Environment, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337 Japan
Search for more papers by this authorCorresponding Author
Dr. Mitsuaki Yamauchi
Department of Applied Chemistry for Environment, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337 Japan
Search for more papers by this authorSeiya Yamamoto
Department of Applied Chemistry for Environment, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337 Japan
Search for more papers by this authorCorresponding Author
Prof. Dr. Sadahiro Masuo
Department of Applied Chemistry for Environment, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337 Japan
Search for more papers by this authorAbstract
Multicomponent supramolecular assembly systems enable the generation of materials with outstanding properties, not obtained from single-component systems, via a synergetic effect. Herein, we demonstrate a novel supramolecular coassembly system rendering highly ordered quantum dot (QD) arrangement structures formed via the self-assembly of azobenzene derivatives, where the photocontrollable photoluminescence (PL) properties of the QDs are realized based on photoisomerization. Upon mixing the assembled azobenzene derivatives and QDs in apolar media, a time-evolution coaggregation into hierarchical nanosheets with a highly ordered QD arrangement structure occurs. Upon photoirradiation, the nanosheets transform into ill-defined aggregates without arranged QDs together with enhancing the PL intensity. In days, the photoirradiated coaggregates undergo recovery of the PL properties corresponding to the arranged QDs through thermal isomerization.
Conflict of interest
The authors declare no conflict of interest.
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