Loading of Exponentially Grown LBL Films with Silver Nanoparticles and Their Application to Generalized SERS Detection†
Sara Abalde-Cela
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorSzushen Ho
Departments of Chemical Engineering, Materials Science and Engineering, and Biomedical Engineering, University of Michigan, Ann Arbor, MI 48109 (USA) http://www.engin.umich.edu/dept/che/research/kotov
Search for more papers by this authorBenito Rodríguez-González Dr.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorMiguel A. Correa-Duarte Dr.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorRamón A. Álvarez-Puebla Dr.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorLuis M. Liz-Marzán Prof.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorNicholas A. Kotov Prof.
Departments of Chemical Engineering, Materials Science and Engineering, and Biomedical Engineering, University of Michigan, Ann Arbor, MI 48109 (USA) http://www.engin.umich.edu/dept/che/research/kotov
Search for more papers by this authorSara Abalde-Cela
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorSzushen Ho
Departments of Chemical Engineering, Materials Science and Engineering, and Biomedical Engineering, University of Michigan, Ann Arbor, MI 48109 (USA) http://www.engin.umich.edu/dept/che/research/kotov
Search for more papers by this authorBenito Rodríguez-González Dr.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorMiguel A. Correa-Duarte Dr.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorRamón A. Álvarez-Puebla Dr.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorLuis M. Liz-Marzán Prof.
Departamento de Química-Física and Unidad Asociada CSIC-Universidade de Vigo, 36310 Vigo (Spain) http://webs.uvigo.es/coloides/nano
Search for more papers by this authorNicholas A. Kotov Prof.
Departments of Chemical Engineering, Materials Science and Engineering, and Biomedical Engineering, University of Michigan, Ann Arbor, MI 48109 (USA) http://www.engin.umich.edu/dept/che/research/kotov
Search for more papers by this authorM.A.C.-D. acknowledges the Isidro Parga Pondal Program fellowship (Xunta de Galicia, Spain) and R.A.A.-P. acknowledges the Ramon y Cajal Program fellowship (Ministerio de Educacion y Ciencia, Spain). This work was funded by the Spanish Ministerio de Ciencia e Innovación (MAT2007-62696 and MAT2008-05755) and the Xunta de Galicia (PGIDIT06TMT31402PR and 08TMT008314PR). We thank A. Benedetti and C. Serra (CACTI, Universidade de Vigo) for carrying out the FIB sample preparation and XPS measurements, respectively. LBL=layer-by-layer; SERS=surface-enhanced Raman scattering.
Abstract
Filmvorstellung: Dünne Filme, die durch exponentielles Schichtenwachstum erzeugt wurden, zeigen hohe Diffusivitäten und lassen sich leicht mit anorganischen Nanopartikeln infiltrieren. Die Filme können molekulare Systeme abhängig von der Schichtzusammensetzung aus Lösungen sequestrieren und liefern oberflächenverstärkte Raman-Signale (SERS) mit hoher Intensität (siehe Bild).
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