Nanoarchitectonics of Metal–Organic Frameworks for Capacitive Deionization via Controlled Pyrolyzed Approaches
Hao Wang
Faculty of Environment and Life, Beijing University of Technology, Beijing, 100124 China
Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL, 60439 USA
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Biaohua Chen
Faculty of Environment and Life, Beijing University of Technology, Beijing, 100124 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
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Di-Jia Liu
Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL, 60439 USA
Pritzker School of Molecular Engineering, The University of Chicago, Chicago, IL, 60637 USA
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
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Xingtao Xu
JST-ERATO Yamauchi Materials Space-Tectonics Project and International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science, Ibaraki, 305-0044 Japan
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorLuigi Osmieri
Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino, 10129 Italy
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Yusuke Yamauchi
Australian Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland, Brisbane, Queensland, 4072 Australia
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorHao Wang
Faculty of Environment and Life, Beijing University of Technology, Beijing, 100124 China
Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL, 60439 USA
Search for more papers by this authorCorresponding Author
Biaohua Chen
Faculty of Environment and Life, Beijing University of Technology, Beijing, 100124 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Di-Jia Liu
Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL, 60439 USA
Pritzker School of Molecular Engineering, The University of Chicago, Chicago, IL, 60637 USA
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Xingtao Xu
JST-ERATO Yamauchi Materials Space-Tectonics Project and International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science, Ibaraki, 305-0044 Japan
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorLuigi Osmieri
Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino, 10129 Italy
Search for more papers by this authorCorresponding Author
Yusuke Yamauchi
Australian Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland, Brisbane, Queensland, 4072 Australia
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorAbstract
Next-generation desalination technologies are needed to meet the increasing demand for clean water. Capacitive deionization (CDI) is a thermodynamically efficient technique to treat non-potable water with relatively low salinity. The salt removal capacity and rate of CDI are highly dependent on the electrode materials, which are preferentially porous to store ions through electrosorption and/or redox reactions. Metal–organic frameworks (MOFs) with “infinite” combinations of transition metals and organic linkers simplify the production of carbonaceous materials often with redox-active components after pyrolysis. MOFs-derived materials show great tunability in both compositions and structures but require further refinement to improve CDI performance. This review article summarizes recent progress in derivatives of MOFs and MOF-like materials used as CDI electrodes, focusing on the structural and compositional material considerations as well as the processing parameters and electrode architectures of the device. Furthermore, the challenges and opportunities associated with this research area are also discussed.
Conflict of Interest
The authors declare no conflict of interest.
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