Review
Phase-Transfer Exchange Lead Chalcogenide Colloidal Quantum Dots: Ink Preparation, Film Assembly, and Solar Cell Construction
Mohan Yuan,
Xia Wang,
Xiao Chen,
Jungang He,
Kanghua Li,
Boxiang Song,
Huicheng Hu,
Liang Gao,
Xinzheng Lan,
Chao Chen,
Jiang Tang,
Mohan Yuan
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorXia Wang
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
Search for more papers by this authorXiao Chen
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
Search for more papers by this authorCorresponding Author
Jungang He
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
E-mail: [email protected], [email protected], [email protected]
Search for more papers by this authorKanghua Li
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorBoxiang Song
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorHuicheng Hu
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorLiang Gao
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorCorresponding Author
Xinzheng Lan
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
E-mail: [email protected], [email protected], [email protected]
Search for more papers by this authorCorresponding Author
Chao Chen
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
E-mail: [email protected], [email protected], [email protected]
Search for more papers by this authorJiang Tang
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorMohan Yuan,
Xia Wang,
Xiao Chen,
Jungang He,
Kanghua Li,
Boxiang Song,
Huicheng Hu,
Liang Gao,
Xinzheng Lan,
Chao Chen,
Jiang Tang,
Mohan Yuan
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorXia Wang
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
Search for more papers by this authorXiao Chen
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
Search for more papers by this authorCorresponding Author
Jungang He
Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China
E-mail: [email protected], [email protected], [email protected]
Search for more papers by this authorKanghua Li
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorBoxiang Song
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorHuicheng Hu
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorLiang Gao
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorCorresponding Author
Xinzheng Lan
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
E-mail: [email protected], [email protected], [email protected]
Search for more papers by this authorCorresponding Author
Chao Chen
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
E-mail: [email protected], [email protected], [email protected]
Search for more papers by this authorJiang Tang
Wuhan National Laboratory for Optoelectronics (WNLO), Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan, Hubei, 430074 P. R. China
Search for more papers by this authorAbstract
Solution-processed colloidal quantum dots (CQDs) are promising candidates for the third-generation photovoltaics due to their low cost and spectral tunability. The development of CQD solar cells mainly relies on high-quality CQD ink, smooth and dense film, and charge-extraction-favored device architectures. In particular, advances in the processing of CQDs are essential for high-quality QD solids. The phase transfer exchange (PTE), in contrast with traditional solid-state ligand exchange, has demonstrated to be the most promising approach for high-quality QD solids in terms of charge transport and defect passivation. As a result, the efficiencies of Pb chalcogenide CQD solar cells have been rapidly improved to 14.0%. In this review, the development of the PTE method is briefly reviewed for lead chalcogenide CQD ink preparation, film assembly, and device construction. Particularly, the key roles of lead halides and additional additives are emphasized for defect passivation and charge transport improvement. In the end, several potential directions for future research are proposed.
Conflict of Interest
The authors declare no conflict of interest.
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