[Ni3(HCOO)6]/Poly(styrene-b-butadiene-b-styrene) Mixed-Matrix Membranes for CH4/N2 Gas Separation
Shumin Wang
Taiyuan University of Technology, College of Materials Science and Engineering, 79, 79, Yingze West Street, 030024 Taiyuan, Shanxi, China
Search for more papers by this authorQingping Guo
Taiyuan University of Technology, College of Materials Science and Engineering, 79, 79, Yingze West Street, 030024 Taiyuan, Shanxi, China
Search for more papers by this authorShujun Liang
Taiyuan Institute of Technology, Department of Materials Engineering, 31, 31, Xinlan Road, 030008 Taiyuan, Shanxi, China
Search for more papers by this authorPeng Li
Taiyuan Institute of Technology, Department of Materials Engineering, 31, 31, Xinlan Road, 030008 Taiyuan, Shanxi, China
Search for more papers by this authorXin Li
Taiyuan Institute of Technology, Department of Materials Engineering, 31, 31, Xinlan Road, 030008 Taiyuan, Shanxi, China
Search for more papers by this authorCorresponding Author
Jujie Luo
Taiyuan University of Technology, College of Materials Science and Engineering, 79, 79, Yingze West Street, 030024 Taiyuan, Shanxi, China
Correspondence: Jujie Luo ([email protected]), Taiyuan University of Technology, College of Materials Science and Engineering, 79, Yingze West Street, Taiyuan, Shanxi 030024, China.Search for more papers by this authorShumin Wang
Taiyuan University of Technology, College of Materials Science and Engineering, 79, 79, Yingze West Street, 030024 Taiyuan, Shanxi, China
Search for more papers by this authorQingping Guo
Taiyuan University of Technology, College of Materials Science and Engineering, 79, 79, Yingze West Street, 030024 Taiyuan, Shanxi, China
Search for more papers by this authorShujun Liang
Taiyuan Institute of Technology, Department of Materials Engineering, 31, 31, Xinlan Road, 030008 Taiyuan, Shanxi, China
Search for more papers by this authorPeng Li
Taiyuan Institute of Technology, Department of Materials Engineering, 31, 31, Xinlan Road, 030008 Taiyuan, Shanxi, China
Search for more papers by this authorXin Li
Taiyuan Institute of Technology, Department of Materials Engineering, 31, 31, Xinlan Road, 030008 Taiyuan, Shanxi, China
Search for more papers by this authorCorresponding Author
Jujie Luo
Taiyuan University of Technology, College of Materials Science and Engineering, 79, 79, Yingze West Street, 030024 Taiyuan, Shanxi, China
Correspondence: Jujie Luo ([email protected]), Taiyuan University of Technology, College of Materials Science and Engineering, 79, Yingze West Street, Taiyuan, Shanxi 030024, China.Search for more papers by this authorAbstract
For the evaluation of CH4/N2 separation, mixed-matrix membranes (MMMs) were fabricated by adding [Ni3(HCOO)6] as a filler into the poly(styrene-b-butadiene-b-styrene) (SBS) polymer. The structures and morphologies of [Ni3(HCOO)6] and [Ni3(HCOO)6]/SBS MMMs were characterized by different techniques, proving the crystalline structure of [Ni3(HCOO)6] in SBS polymer matrices. The structural integrity of the MMMs and good compatibility between [Ni3(HCOO)6] and SBS polymer were examined by scanning electron microscopy. Gas permeation measurements revealed that membranes containing various [Ni3(HCOO)6] loadings exhibited different separation performances. The operational temperature exerted a significantly positive effect on the separation of CH4 and N2.
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