Methods for the Trace Oxygen Removal from Methane-Rich Gas Streams
Tim Peppel
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.
Search for more papers by this authorDominik Seeburg
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.
Search for more papers by this authorGerhard Fulda
Medical Biology and Electron Microscopy Centre, University Medicine, Strempelstrasse 14, 18057 Rostock Germany.
Search for more papers by this authorMarkus Kraus
Department of Environmental Engineering, Helmholtz Centre for Environmental Research – UFZ, Permoserstrasse 15, 04318 Leipzig, Germany.
Search for more papers by this authorUlf Trommler
Department of Environmental Engineering, Helmholtz Centre for Environmental Research – UFZ, Permoserstrasse 15, 04318 Leipzig, Germany.
Search for more papers by this authorUlf Roland
Department of Environmental Engineering, Helmholtz Centre for Environmental Research – UFZ, Permoserstrasse 15, 04318 Leipzig, Germany.
Search for more papers by this authorCorresponding Author
Sebastian Wohlrab
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.Search for more papers by this authorTim Peppel
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.
Search for more papers by this authorDominik Seeburg
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.
Search for more papers by this authorGerhard Fulda
Medical Biology and Electron Microscopy Centre, University Medicine, Strempelstrasse 14, 18057 Rostock Germany.
Search for more papers by this authorMarkus Kraus
Department of Environmental Engineering, Helmholtz Centre for Environmental Research – UFZ, Permoserstrasse 15, 04318 Leipzig, Germany.
Search for more papers by this authorUlf Trommler
Department of Environmental Engineering, Helmholtz Centre for Environmental Research – UFZ, Permoserstrasse 15, 04318 Leipzig, Germany.
Search for more papers by this authorUlf Roland
Department of Environmental Engineering, Helmholtz Centre for Environmental Research – UFZ, Permoserstrasse 15, 04318 Leipzig, Germany.
Search for more papers by this authorCorresponding Author
Sebastian Wohlrab
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.
Leibniz Institute for Catalysis at the University of Rostock, Albert-Einstein-Strasse 29a, 18059 Rostock, Germany.Search for more papers by this authorAbstract
Oxygen removal to very low residual contents in methane-rich gas streams and carbon dioxide as co-component (simulated biogas) was achieved via three different methods at various temperatures, namely, by reduction with hydrogen admixtures on Pt/γ-Al2O3 catalysts, by oxygen absorption affinity of YBaCo4O7+δ, and by the catalytic reaction with methane on both the materials, respectively. The three methods have characteristic advantages and disadvantages which are discussed in the context of existing methods for gas treatments focused on oxygen removal. Finally, the advantage of dielectric radio-frequency heating on the powdered functional materials is suggested as alternative to conventional routes.
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