Superconducting Double Perovskite Bismuth Oxide Prepared by a Low-Temperature Hydrothermal Reaction
Mirza H. K. Rubel
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Akira Miura
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Takahiro Takei
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorCorresponding Author
Prof. Nobuhiro Kumada
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)Search for more papers by this authorM. Mozahar Ali
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Masanori Nagao
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Satoshi Watauchi
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Isao Tanaka
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Kengo Oka
Materials and Structural laboratory, Tokyo Institute of Technology, 4259 Nagatsuta, Midori-ku Yokohama-city, Kanagawa 226-8503 (Japan)
Search for more papers by this authorProf. Masaki Azuma
Materials and Structural laboratory, Tokyo Institute of Technology, 4259 Nagatsuta, Midori-ku Yokohama-city, Kanagawa 226-8503 (Japan)
Search for more papers by this authorProf. Eisuke Magome
Department of Physical Science, Hiroshima University, 1-3-1 Kagamiyama, Higashihiroshima, Hiroshima 739-8526 (Japan)
Search for more papers by this authorProf. Chikako Moriyoshi
Department of Physical Science, Hiroshima University, 1-3-1 Kagamiyama, Higashihiroshima, Hiroshima 739-8526 (Japan)
Search for more papers by this authorProf. Yoshihiro Kuroiwa
Department of Physical Science, Hiroshima University, 1-3-1 Kagamiyama, Higashihiroshima, Hiroshima 739-8526 (Japan)
Search for more papers by this authorProf. A. K. M. Azharul Islam
Department of Physics, University of Rajshahi, Rajshahi-6205 (Bangladesh)
Search for more papers by this authorMirza H. K. Rubel
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Akira Miura
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Takahiro Takei
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorCorresponding Author
Prof. Nobuhiro Kumada
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)Search for more papers by this authorM. Mozahar Ali
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Masanori Nagao
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Satoshi Watauchi
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Isao Tanaka
Center for Crystal Science and Technology, University of Yamanashi, 7-32 Miyamae Kofu 400-8511 (Japan)
Search for more papers by this authorProf. Kengo Oka
Materials and Structural laboratory, Tokyo Institute of Technology, 4259 Nagatsuta, Midori-ku Yokohama-city, Kanagawa 226-8503 (Japan)
Search for more papers by this authorProf. Masaki Azuma
Materials and Structural laboratory, Tokyo Institute of Technology, 4259 Nagatsuta, Midori-ku Yokohama-city, Kanagawa 226-8503 (Japan)
Search for more papers by this authorProf. Eisuke Magome
Department of Physical Science, Hiroshima University, 1-3-1 Kagamiyama, Higashihiroshima, Hiroshima 739-8526 (Japan)
Search for more papers by this authorProf. Chikako Moriyoshi
Department of Physical Science, Hiroshima University, 1-3-1 Kagamiyama, Higashihiroshima, Hiroshima 739-8526 (Japan)
Search for more papers by this authorProf. Yoshihiro Kuroiwa
Department of Physical Science, Hiroshima University, 1-3-1 Kagamiyama, Higashihiroshima, Hiroshima 739-8526 (Japan)
Search for more papers by this authorProf. A. K. M. Azharul Islam
Department of Physics, University of Rajshahi, Rajshahi-6205 (Bangladesh)
Search for more papers by this authorGraphical Abstract
A double helping: The title compound was prepared by hydrothermal reaction of NaBiO3⋅n H2O, Ba(OH)2⋅8 H2O, and KOH at 220 °C. The structure of the double perovskite was determined to be (Na0.25K0.45)(Ba1.00)3(Bi1.00)4O12, and thermally decomposed to a simple perovskite structure above 400 °C. The synthesized compounds exhibit superconductive diamagnetism, and zero resistivity below 8 K.
Abstract
Perovskite-type structures (ABO3) have received significant attention because of their crystallographic aspects and physical properties, but there has been no clear evidence of a superconductor with a double-perovskite-type structure, whose different elements occupy A and/or B sites in ordered ways. In this report, hydrothermal synthesis at 220 °C produced a new superconductor with an A-site-ordered double perovskite structure, (Na0.25K0.45)(Ba1.00)3(Bi1.00)4O12, with a maximum Tc of about 27 K.
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