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Innenrücktitelbild: The Redox Coupling Effect in a Photocatalytic Ru^II-Pd^II Cage with TTF Guest as Electron Relay Mediator for Visible-Light Hydrogen-Evolving Promotion (Angew. Chem. 7/2020)

Dr. Kai Wu

orcid.org/0000-0001-6336-7836

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

These authors contributed equally to this work.

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Dr. Kang Li,

Dr. Kang Li

orcid.org/0000-0003-2533-1829

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

These authors contributed equally to this work.

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Dr. Sha Chen,

Dr. Sha Chen

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Dr. Ya-Jun Hou,

Dr. Ya-Jun Hou

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Yu-Lin Lu,

Yu-Lin Lu

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Jing-Si Wang,

Jing-Si Wang

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Mei-Juan Wei,

Mei-Juan Wei

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Prof. Dr. Mei Pan,

Prof. Dr. Mei Pan

orcid.org/0000-0002-8979-7305

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Prof. Dr. Cheng-Yong Su,

Corresponding Author

Prof. Dr. Cheng-Yong Su

[email protected]

orcid.org/0000-0003-3604-7858

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, China

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Dr. Kai Wu,

Dr. Kai Wu

orcid.org/0000-0001-6336-7836

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

These authors contributed equally to this work.

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Dr. Kang Li,

Dr. Kang Li

orcid.org/0000-0003-2533-1829

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

These authors contributed equally to this work.

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Dr. Sha Chen,

Dr. Sha Chen

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Dr. Ya-Jun Hou,

Dr. Ya-Jun Hou

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Yu-Lin Lu,

Yu-Lin Lu

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Jing-Si Wang,

Jing-Si Wang

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Mei-Juan Wei,

Mei-Juan Wei

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Prof. Dr. Mei Pan,

Prof. Dr. Mei Pan

orcid.org/0000-0002-8979-7305

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

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Prof. Dr. Cheng-Yong Su,

Corresponding Author

Prof. Dr. Cheng-Yong Su

[email protected]

orcid.org/0000-0003-3604-7858

MOE Laboratory of Bioinorganic and Synthetic Chemistry, Lehn Institute of Functional Materials, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275 China

State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, China

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First published: 22 January 2020

https://doi.org/10.1002/ange.202000295

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Graphical Abstract

Ein Nanospace-Kopplungseffekt in einem photokatalytischen Ru^II-Pd^II-Käfig basiert auf dem Redox-Wechselspiel zwischen einem TTF-Gastmolekül und dem photosensibilisierenden Wirt in der H₂-Entwicklung mit sichtbarem Licht. Wie C.-Y. Su und Mitarbeiter in ihrer Zuschrift auf S. 2661 beschreiben, fungiert der TTF-Gast als Elektronenrelais, indem er durch Kopplung mit dem Photoredoxzyklus des Käfigs den Elektronentransferprozess moduliert, was zu einer signifikanten Verbesserung der Wasserstoffentwicklungseffizienz führt.