Active Water Optimization in Different Electrolyte Systems for Stable Zinc Anodes
Guoxing Tian
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorCorresponding Author
Ailing Song
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorMing Liu
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorYanan Song
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorYing Liu
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorNingning Tian
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorYuqian Fan
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorCorresponding Author
Ling Chen
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Guangjie Shao
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Zhipeng Ma
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorGuoxing Tian
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorCorresponding Author
Ailing Song
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorMing Liu
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorYanan Song
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorYing Liu
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorNingning Tian
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorYuqian Fan
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
Search for more papers by this authorCorresponding Author
Ling Chen
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Guangjie Shao
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Zhipeng Ma
Hebei Key Laboratory of Applied Chemistry, College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, 066004 China
State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao, 066004 China
E-mail: [email protected]; [email protected]; [email protected]; [email protected]
Search for more papers by this authorAbstract
Zinc (Zn) metal, with abundant resources, intrinsic safety, and environmental benignity, presents an attractive prospect as a novel electrode material. However, many substantial challenges remain in realizing the widespread application of aqueous Zn-ion batteries (AZIBs) technologies. These encompass significant material corrosion challenges (This can lead to battery failure in an unloaded state.), hydrogen evolution reactions, pronounced dendrite growth at the anode interface, and a constrained electrochemical stability window. Consequently, these factors contribute to diminished battery lifespan and energy efficiency while restricting high-voltage performance. Although numerous reviews have addressed the potential of electrode and separator design to mitigate these issues to some extent, the inherent reactivity of water remains the fundamental source of these challenges, underscoring the necessity for precise regulation of active water molecules within the electrolyte. In this review, the failure mechanism of AZIBs (unloaded and in charge and discharge state) is analyzed, and the optimization strategy and working principle of water in the electrolyte are reviewed, aiming to provide insights for effectively controlling the corrosion process and hydrogen evolution reaction, further controlling dendrite formation, and expanding the range of electrochemical stability. Furthermore, it outlines the challenges to promote its practical application and future development pathways.
Conflict of Interest
The authors declare no conflict of interest.
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