Review
Progress of Polymer Electrolytes Worked in Solid-State Lithium Batteries for Wide-Temperature Application
Long Hu,
Xue Gao,
Hui Wang,
Yun Song,
Yongli Zhu,
Zhijun Tao,
Bin Yuan,
Renzong Hu,
Long Hu
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Search for more papers by this authorXue Gao
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Search for more papers by this authorHui Wang
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Search for more papers by this authorCorresponding Author
Yun Song
Department of Materials Science, Fudan University, Shanghai, 200433 China
E-mail: [email protected]; [email protected]
Search for more papers by this authorYongli Zhu
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Search for more papers by this authorZhijun Tao
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Search for more papers by this authorBin Yuan
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Search for more papers by this authorCorresponding Author
Renzong Hu
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Institute of Science and Technology for New Energy, Xi'an Technological University, Xi'an, 710021 China
E-mail: [email protected]; [email protected]
Search for more papers by this authorLong Hu,
Xue Gao,
Hui Wang,
Yun Song,
Yongli Zhu,
Zhijun Tao,
Bin Yuan,
Renzong Hu,
Long Hu
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Search for more papers by this authorXue Gao
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Search for more papers by this authorHui Wang
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Search for more papers by this authorCorresponding Author
Yun Song
Department of Materials Science, Fudan University, Shanghai, 200433 China
E-mail: [email protected]; [email protected]
Search for more papers by this authorYongli Zhu
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Search for more papers by this authorZhijun Tao
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Search for more papers by this authorBin Yuan
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Search for more papers by this authorCorresponding Author
Renzong Hu
School of Materials Science and Engineering, Guangdong Engineering Technology Research Center of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510641 China
Guangdong Huajing New Energy Technology Co. Ltd, Foshan, 528313 China
Institute of Science and Technology for New Energy, Xi'an Technological University, Xi'an, 710021 China
E-mail: [email protected]; [email protected]
Search for more papers by this authorAbstract
Solid-state Li-ion batteries have emerged as the most promising next-generation energy storage systems, offering theoretical advantages such as superior safety and higher energy density. However, polymer-based solid-state Li-ion batteries face challenges across wide temperature ranges. The primary issue lies in the fact that most polymer electrolytes exhibit relatively low ionic conductivity at or below room temperature. This sensitivity to temperature variations poses challenges in operating solid-state lithium batteries at sub-zero temperatures. Moreover, elevated working temperatures lead to polymer shrinkage and deformation, ultimately resulting in battery failure. To address this challenge of polymer-based solid-state batteries, this review presents an overview of various promising polymer electrolyte systems. The review provides insights into the temperature-dependent physical and electrochemical properties of polymers, aiming to expand the temperature range of operation. The review also further summarizes modification strategies for polymer electrolytes suited to diverse temperatures. The final section summarizes the performance of various polymer-based solid-state batteries at different temperatures. Valuable insights and potential future research directions for designing wide-temperature polymer electrolytes are presented based on the differences in battery performance. This information is intended to inspire practical applications of wide-temperature polymer-based solid-state batteries.
Conflict of Interest
The authors declare no conflict of interest.
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