Temperature effect and kinetics, LiZr2(PO4)3 and Li1.2Al0.2Zr1.8(PO4)3 and electrochemical properties for rechargeable ion batteries
Bhargav Akkinepally
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
School of General Education, Yeungnam University, Gyeongsan, Republic of Korea
Bhargav Akkinepally and I. Neelakanta Reddy contributed equally to this work.
Search for more papers by this authorCorresponding Author
I. Neelakanta Reddy
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
Bhargav Akkinepally and I. Neelakanta Reddy contributed equally to this work.
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorV. Manjunath
Department of Physics, Sri Padmavati Mahila Visvavidyalayam, Tirupati, India
Search for more papers by this authorCorresponding Author
M. V. Reddy
Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Yogendra Kumar Mishra
Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Tae Jo Ko
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Karim Zaghib
Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Jaesool Shim
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorBhargav Akkinepally
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
School of General Education, Yeungnam University, Gyeongsan, Republic of Korea
Bhargav Akkinepally and I. Neelakanta Reddy contributed equally to this work.
Search for more papers by this authorCorresponding Author
I. Neelakanta Reddy
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
Bhargav Akkinepally and I. Neelakanta Reddy contributed equally to this work.
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorV. Manjunath
Department of Physics, Sri Padmavati Mahila Visvavidyalayam, Tirupati, India
Search for more papers by this authorCorresponding Author
M. V. Reddy
Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Yogendra Kumar Mishra
Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Tae Jo Ko
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Karim Zaghib
Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorCorresponding Author
Jaesool Shim
School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea
Correspondence
I. Neelakanta Reddy, Tae Jo Ko and Jaesool Shim, School of Mechanical Engineering, Yeungnam University, Gyeongsan, Republic of Korea.
Email: [email protected], [email protected] and [email protected]
M. V. Reddy, Nouveau Monde Graphite, Saint-Michel-de-Saints, Canada.
Email: [email protected]
Yogendra Kumar Mishra, Mads Clausen Institute, NanoSYD, University of Southern Denmark, Sønderborg, Denmark.
Email: [email protected]
Karim Zaghib, Department of Chemical and Materials Engineering, Concordia University, Montréal, Canada.
Email: [email protected]
Search for more papers by this authorFunding information: National Research Foundation, Grant/Award Numbers: 2020R1A2C1012439, 2020R1A4A1019227
Summary
A NASICON-type LiZr2(PO4)3 (LZP) and Li1.2Al0.2Zr1.8(PO4)3 (LAZP) anode materials are synthesized via a facile method, materials were characterized by a variety of structural techniques, investigated the electrochemical performance for rechargeable battery applications. A highly stable rhombohedral phase of LAZP is noticed at room temperature, with a discharge capacity of 909 mAh.g−1, which is 1.6 times higher than that of LZP. Further, the highly stable charge storage performance is observed up to 3000 cycles with a Coulombic efficiency of 99%. For the first time, we investigated the in-situ temperature effect on the discharge capacity of the assembled anode material, found a strong effect on the discharge capacity, and achieved ~120 and 149 mAh.g−1 at 65°C for LZP and LAZP anodes. Furthermore, the real-time charge holding effect of LAZP cell is performed with the computer, the cell worked well in the CMOS battery slot without a CMOS battery error during CPU turn-on condition for 1536 h. In brief, an optimized electrode material of LAZP showed greater stability and capacity with high efficiency compared with LZP even at elevated temperatures. Hence, LAZP may be utilized to fabricate a coin cell for real time applications.
Open Research
DATA AVAILABILITY STATEMENT
The data that support the findings of this study are available from the corresponding author upon reasonable request.
Supporting Information
| Filename | Description |
|---|---|
| er8129-sup-0001-Supinfo.docxWord 2007 document , 4.1 MB | Appendix S1 |
| er8129-sup-0002-VideoS1.aviAVI video, 13.6 MB | Video S1 |
Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.
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