Volume 8, Issue 3 1901111

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Fabrication of Graphene Oxide Supported Acid–Base Bifunctional Metal–Organic Frameworks as Efficient Catalyst for Glucose to 5-Hydroxymethylfurfural Conversion

Yanan Wei

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Yunlei Zhang,

Corresponding Author

Yunlei Zhang

[email protected]

orcid.org/0000-0003-3536-9142

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Bing Li,

Bing Li

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Changhao Yan,

Changhao Yan

Research Center of Fluid Machinery Engineering and Technology, Jiangsu University, Zhenjiang, 212000 P. R. China

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Zulin Da,

Zulin Da

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Minjia Meng,

Minjia Meng

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Chunbo Liu,

Chunbo Liu

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Yongsheng Yan,

Corresponding Author

Yongsheng Yan

[email protected]

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Yanan Wei,

Yanan Wei

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Yunlei Zhang,

Corresponding Author

Yunlei Zhang

[email protected]

orcid.org/0000-0003-3536-9142

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Bing Li,

Bing Li

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Changhao Yan,

Changhao Yan

Research Center of Fluid Machinery Engineering and Technology, Jiangsu University, Zhenjiang, 212000 P. R. China

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Zulin Da,

Zulin Da

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Minjia Meng,

Minjia Meng

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Chunbo Liu,

Chunbo Liu

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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Yongsheng Yan,

Corresponding Author

Yongsheng Yan

[email protected]

Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212000 P. R. China

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First published: 09 January 2020

https://doi.org/10.1002/ente.201901111

Citations: 23

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Abstract

Developing a supported-type metal–organic frameworks (MOFs) catalyst with multifunctional active sites is essential to broaden its application as a heterogeneous catalyst. Herein, polydopamine (PDA)-modified graphene oxide (PDA@GO) is used as a support to prepare an acid–base bifunctional UiO-66-type MOFs catalyst in green solution (aqueous solution) through a one-pot method. By adjusting the amount between GO, PDA, UiO-66-NH₂, and UiO-66-SO₃H, the heterogeneous solid catalyst UiO-66-SO₃H-NH₂/PDA@GO with uniform distribution of MOFs can be obtained. The morphology and various properties of the catalyst are characterized and the catalytic performance of the catalyst for the conversion of glucose to 5-hydroxymethylfurfural (5-HMF) is demonstrated and discussed. Herein, the supported-type MOFs catalyst offers an alternative way to promote current acid–base catalytic systems for achieving efficient production of 5-HMF from sustainable biomass.

Conflict of Interest

The authors declare no conflict of interest.

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Volume8, Issue3

March 2020

1901111

Fabrication of Graphene Oxide Supported Acid–Base Bifunctional Metal–Organic Frameworks as Efficient Catalyst for Glucose to 5-Hydroxymethylfurfural Conversion

Abstract

Conflict of Interest

References

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Fabrication of Graphene Oxide Supported Acid–Base Bifunctional Metal–Organic Frameworks as Efficient Catalyst for Glucose to 5-Hydroxymethylfurfural Conversion

Abstract

Conflict of Interest

References

Citing Literature

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