Waste organic acid treatment with polyethyleneimine grafted polystyrene resin
Qi Meng
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Conceptualization (lead), Funding acquisition (supporting), Investigation (equal), Project administration (equal), Writing - original draft (equal)
Search for more papers by this authorYiwen Cao
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Investigation (equal), Methodology (equal), Writing - original draft (equal)
Search for more papers by this authorShufeng Ma
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Investigation (equal)
Search for more papers by this authorMeiling Wang
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Software (supporting), Validation (supporting)
Search for more papers by this authorHao Niu
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Software (supporting), Validation (supporting)
Search for more papers by this authorWeihua Jiang
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Resources (equal)
Search for more papers by this authorCorresponding Author
Qiaoqiao Teng
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Correspondence
Qiaoqiao Teng, Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, 213164, China.
Email: [email protected]
Ninghong Jia, State Key Laboratory of Enhanced Oil Recovery, Research Institute of Petroleum Exploration & Development, Beijing, 100083, China.
Email: [email protected]
Contribution: Conceptualization (equal), Funding acquisition (lead), Project administration (lead), Supervision (lead)
Search for more papers by this authorCorresponding Author
Ninghong Jia
State Key Laboratory of Enhanced Oil Recovery, Research Institute of Petroleum Exploration & Development, Beijing, China
Correspondence
Qiaoqiao Teng, Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, 213164, China.
Email: [email protected]
Ninghong Jia, State Key Laboratory of Enhanced Oil Recovery, Research Institute of Petroleum Exploration & Development, Beijing, 100083, China.
Email: [email protected]
Contribution: Resources (lead), Supervision (equal)
Search for more papers by this authorQi Meng
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Conceptualization (lead), Funding acquisition (supporting), Investigation (equal), Project administration (equal), Writing - original draft (equal)
Search for more papers by this authorYiwen Cao
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Investigation (equal), Methodology (equal), Writing - original draft (equal)
Search for more papers by this authorShufeng Ma
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Investigation (equal)
Search for more papers by this authorMeiling Wang
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Software (supporting), Validation (supporting)
Search for more papers by this authorHao Niu
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Software (supporting), Validation (supporting)
Search for more papers by this authorWeihua Jiang
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Contribution: Resources (equal)
Search for more papers by this authorCorresponding Author
Qiaoqiao Teng
Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, China
Correspondence
Qiaoqiao Teng, Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, 213164, China.
Email: [email protected]
Ninghong Jia, State Key Laboratory of Enhanced Oil Recovery, Research Institute of Petroleum Exploration & Development, Beijing, 100083, China.
Email: [email protected]
Contribution: Conceptualization (equal), Funding acquisition (lead), Project administration (lead), Supervision (lead)
Search for more papers by this authorCorresponding Author
Ninghong Jia
State Key Laboratory of Enhanced Oil Recovery, Research Institute of Petroleum Exploration & Development, Beijing, China
Correspondence
Qiaoqiao Teng, Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou, 213164, China.
Email: [email protected]
Ninghong Jia, State Key Laboratory of Enhanced Oil Recovery, Research Institute of Petroleum Exploration & Development, Beijing, 100083, China.
Email: [email protected]
Contribution: Resources (lead), Supervision (equal)
Search for more papers by this authorFunding information: CNPC Innovation Found, Grant/Award Number: 2021DQ02-1104; Graduate Research and Innovation Projects of Jiangsu Province, Grant/Award Number: SJCX21_1218; Jiangsu Key Laboratory of Fine Petrochemical Engineering, Grant/Award Number: KF2005; National Natural Science Foundation of China, Grant/Award Number: 22001022
Abstract
Organic acid is a kind of important fine chemicals with wide application, while impropriate discharges would cause serious damage to environment. In this report, two polyethyleneimine (PEI-600, 1800) functionalized polystyrene (PS) resins were facilely prepared to remediate common organic acids. The heavier PEI-1800 resulted in surprisingly lower nitrogen loading of PSPEI under optimal conditions due to more significant extra grafting. Therefore, PSPEI-600 was used to adsorb two groups (aliphatic and aromatic) of eight common organic acids, and showed highest adsorptive capacities toward salicylic acid (SA) and trifluoroacetic acid (TFA). The adsorption of TFA was faster and was mainly due to strong acid–base interactions by forming ammonium carboxylate. SA possessed lower acidity, but its additional π-π stacking and hydrogen bonding interactions with the PSPEI resin led to a slower but overall higher uptake. Kinetic studies indicated that both acid adsorptions conformed to pseudo-second-order kinetics, and the adsorption rate was controlled by intraparticle diffusion. The adsorptions followed Langmuir isotherms and were identified as a spontaneous endothermic process.
CONFLICT OF INTEREST
We declare that we do not have any commercial or associative interest that represents a conflict of interest in connection with the work submitted.
Open Research
DATA AVAILABILITY STATEMENT
The data sets generated during the current study are available in the supporting information.
Supporting Information
| Filename | Description |
|---|---|
| app53433-sup-0001-Supinfo.docxWord 2007 document , 116 KB | Appendix S1: Supporting Information |
Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.
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