Photocatalytic Conversion of Methane: Recent Advancements and Prospects
Qi Li
State Key Laboratory for Powder Metallurgy, School of Materials Science and Engineering, Central South University, Changsha, Hunan, 410083 P. R. China
Search for more papers by this authorYuxing Ouyang
State Key Laboratory for Powder Metallurgy, School of Materials Science and Engineering, Central South University, Changsha, Hunan, 410083 P. R. China
Search for more papers by this authorDr. Hongliang Li
Hefei National Laboratory for Physical Sciences at the Microscale, Key Laboratory of Strongly-Coupled Quantum Matter Physics of Chinese Academy of Sciences, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China, Hefei, Anhui, 230026 P. R. China
Search for more papers by this authorCorresponding Author
Prof. Liangbing Wang
State Key Laboratory for Powder Metallurgy, School of Materials Science and Engineering, Central South University, Changsha, Hunan, 410083 P. R. China
Search for more papers by this authorCorresponding Author
Prof. Jie Zeng
Hefei National Laboratory for Physical Sciences at the Microscale, Key Laboratory of Strongly-Coupled Quantum Matter Physics of Chinese Academy of Sciences, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China, Hefei, Anhui, 230026 P. R. China
Search for more papers by this authorQi Li
State Key Laboratory for Powder Metallurgy, School of Materials Science and Engineering, Central South University, Changsha, Hunan, 410083 P. R. China
Search for more papers by this authorYuxing Ouyang
State Key Laboratory for Powder Metallurgy, School of Materials Science and Engineering, Central South University, Changsha, Hunan, 410083 P. R. China
Search for more papers by this authorDr. Hongliang Li
Hefei National Laboratory for Physical Sciences at the Microscale, Key Laboratory of Strongly-Coupled Quantum Matter Physics of Chinese Academy of Sciences, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China, Hefei, Anhui, 230026 P. R. China
Search for more papers by this authorCorresponding Author
Prof. Liangbing Wang
State Key Laboratory for Powder Metallurgy, School of Materials Science and Engineering, Central South University, Changsha, Hunan, 410083 P. R. China
Search for more papers by this authorCorresponding Author
Prof. Jie Zeng
Hefei National Laboratory for Physical Sciences at the Microscale, Key Laboratory of Strongly-Coupled Quantum Matter Physics of Chinese Academy of Sciences, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China, Hefei, Anhui, 230026 P. R. China
Search for more papers by this authorGraphical Abstract
The conversion of methane driven by solar energy offers a promising approach to directly transform methane into valuable energy sources under mild conditions, but remains a great challenge. This Review highlights recent advances in the photocatalytic conversion of methane and gives insights into the design of effective semiconductor-based photocatalysts and classifies the photooxidations according to the oxidants in the reaction system.
Abstract
Abundant and affordable methane is not only a high-quality fossil fuel, it is also a raw material for the synthesis of value-added chemicals. Solar-energy-driven conversion of methane offers a promising approach to directly transform methane to valuable energy sources under mild conditions, but remains a great challenge at present. In this Review, recent advances in the photocatalytic conversion of methane are systematically summarized. Insights into the construction of effective semiconductor-based photocatalysts from the perspective of light-absorption units and active centers are highlighted and discussed in detail. The performance of various photocatalysts in the conversion of methane is presented, with the photooxidation classified according to the oxidant systems. Lastly, challenges and future perspectives in the photocatalytic oxidation of methane are described.
Conflict of interest
The authors declare no conflict of interest.
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