Volume 48, Issue 22 pp. 3987-3990

Communication

Highly Selective Catalytic Conversion of Phenolic Bio-Oil to Alkanes^†

Chen Zhao,

Chen Zhao

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

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Yuan Kou Prof. Dr.,

Yuan Kou Prof. Dr.

[email protected]

PKU Green Chemistry Center, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871 (China), Fax: (+86) 10-6275-1708

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Angeliki A. Lemonidou Prof. Dr.,

Angeliki A. Lemonidou Prof. Dr.

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

Permanent address: Department of Chemical Engineering, Aristotle University of Thessaloniki (Greece)

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Xuebing Li Dr.,

Xuebing Li Dr.

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

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Johannes A. Lercher Prof. Dr.,

Johannes A. Lercher Prof. Dr.

[email protected]

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

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Chen Zhao,

Chen Zhao

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

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Yuan Kou Prof. Dr.,

Yuan Kou Prof. Dr.

[email protected]

PKU Green Chemistry Center, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871 (China), Fax: (+86) 10-6275-1708

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Angeliki A. Lemonidou Prof. Dr.,

Angeliki A. Lemonidou Prof. Dr.

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

Permanent address: Department of Chemical Engineering, Aristotle University of Thessaloniki (Greece)

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Xuebing Li Dr.,

Xuebing Li Dr.

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

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Johannes A. Lercher Prof. Dr.,

Johannes A. Lercher Prof. Dr.

[email protected]

Department Chemie, Technische Universität München, 85747 Garching (Germany), Fax: (+49) 89-2891-3544

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First published: 12 May 2009

https://doi.org/10.1002/anie.200900404

Citations: 595

^†

This research was performed in the framework of the Network of Excellence IDECAT.

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Graphical Abstract

Oil and water: A new energy-efficient and atom-economical catalytic route for the production of alkanes and methanol by upgrading the phenolic fraction of bio-oil has been developed. The one-pot aqueous-phase hydrodeoxygenation process is based on two catalysts facilitating consecutive hydrogenation, hydrolysis, and dehydration reactions.

Abstract

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References

1E. Furimsky, Appl. Catal. A 2000, 199, 147–190.
10.1016/S0926-860X(99)00555-4
CAS Web of Science® Google Scholar
2S. Czernik, A. V. Bridgwater, Energy Fuels 2004, 18, 590–598.
10.1021/ef034067u
CAS Web of Science® Google Scholar
3G. W. Huber, S. Iborra, A. Corma, Chem. Rev. 2006, 106, 4044–4098.
10.1021/cr068360d
CAS PubMed Web of Science® Google Scholar
4
4aE. G. Baker, D. C. Elliott, US Patent, 5,180,868, 1993;
Google Scholar
4bE. Laurent, B. Delmon, J. Catal. 1994, 146, 281–291;
10.1016/0021-9517(94)90032-9
CAS Web of Science® Google Scholar
4cA. Centeno, E. Laurent, B. Delmon, J. Catal. 1995, 154, 288–298;
10.1006/jcat.1995.1170
CAS Web of Science® Google Scholar
4dE. Furimsky, F. E. Massoth, Catal. Today 1999, 52, 381–495;
10.1016/S0920-5861(99)00096-6
CAS Web of Science® Google Scholar
4eJ. S. Shabtai, W. W. Zmierczak, E. Chornet, US Patent, 5,959,167, 1999;
Google Scholar
4fT. R. Viljava, R. S. Komulanien, A. O. I. Krause, Catal. Today 2000, 60, 83–92.
10.1016/S0920-5861(00)00320-5
CAS Web of Science® Google Scholar
5
5aR. D. Cortright, R. R. Davda, J. A. Dumesic, Nature 2002, 418, 964–967;
10.1038/nature01009
CAS PubMed Web of Science® Google Scholar
5bG. W. Huber, J. W. Shabaker, J. A. Dumesic, Science 2003, 300, 2075–2077;
10.1126/science.1085597
CAS PubMed Web of Science® Google Scholar
5cG. W. Huber, R. D. Cortright, J. A. Dumesic, Angew. Chem. 2004, 116, 1575–1577;
10.1002/ange.200353050
Web of Science® Google Scholar
Angew. Chem. Int. Ed. 2004, 43, 1549–1551;
10.1002/anie.200353050
CAS PubMed Web of Science® Google Scholar
5dR. R. Soares, D. A. Simonetti, J. A. Dumesic, Angew. Chem. 2006, 118, 4086–4089;
10.1002/ange.200600212
Google Scholar
Angew. Chem. Int. Ed. 2006, 45, 3982–3985;
10.1002/anie.200600212
CAS PubMed Web of Science® Google Scholar
5eN. Yan, C. Zhao, C. Luo, P. J. Dyson, H. Liu, Y. Kou, J. Am. Chem. Soc. 2006, 128, 8714–8715.
10.1021/ja062468t
CAS PubMed Web of Science® Google Scholar
6C. Zhao, W. J. Gan, X. B. Fan, Z. P. Cai, P. J. Dyson, Y. Kou, J. Catal. 2008, 254, 244–250.
10.1016/j.jcat.2008.01.003
CAS Web of Science® Google Scholar
7T. Wang, C. X. Xiao, L. Yan, L. Xu, J. Luo, H. Shou, Y. Kou, H. Liu, Chem. Commun. 2007, 4375–4377.
10.1039/b710845a
CAS PubMed Web of Science® Google Scholar
8C. X. Xiao, Z. P. Cai, T. Wang, Y. Kou, N. Yan, Angew. Chem. 2008, 120, 758–761;
10.1002/ange.200703481
Web of Science® Google Scholar
Angew. Chem. Int. Ed. 2008, 47, 746–749.
10.1002/anie.200703481
CAS PubMed Web of Science® Google Scholar
9
9aA. K. Talukdar, K. G. Bhattacharyya, Appl. Catal. A 1993, 96, 229–239;
10.1016/0926-860X(90)80012-4
CAS Web of Science® Google Scholar
9bG. Neri, A. M. Visco, A. Donato, C. Milone, M. Malentacchi, G. Gubitosa, Appl. Catal. A 1994, 110, 49–59;
10.1016/0926-860X(94)80104-5
CAS Web of Science® Google Scholar
9cN. Mahata, V. Vishwanathan, J. Catal. 2000, 196, 262–270;
10.1006/jcat.2000.3041
CAS Web of Science® Google Scholar
9dS. Scirè, S. Minico, C. Crisafulli, Appl. Catal. A 2002, 235, 21–31;
10.1016/S0926-860X(02)00237-5
CAS Web of Science® Google Scholar
9eE. Díaz, A. F. Mohedano, L. Calvo, M. A. Gilarranz, J. A. Casas, J. J. Rodríguez, Chem. Eng. J. 2007, 131, 65–71;
10.1016/j.cej.2006.12.020
CAS Web of Science® Google Scholar
9fG. Yuan, M. A. Keane, Ind. Eng. Chem. Res. 2007, 46, 705–715;
10.1021/ie060802o
CAS Web of Science® Google Scholar
9gY. Z. Xiang, L. Ma, C. S. Lu, Q. F. Zhang, X. N. Li, Green Chem. 2008, 10, 939–943.
10.1039/b803217c
CAS Web of Science® Google Scholar
10D. C. Elliott, Energy Fuels 2007, 21, 1792–1815.
10.1021/ef070044u
CAS Web of Science® Google Scholar
11M. J. Girgis, B. C. Gates, Ind. Eng. Chem. Res. 1991, 30, 2021–2058.
10.1021/ie00057a001
CAS Web of Science® Google Scholar

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Volume48, Issue22

May 18, 2009

Pages 3987-3990

Highly Selective Catalytic Conversion of Phenolic Bio-Oil to Alkanes^†

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Abstract

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Highly Selective Catalytic Conversion of Phenolic Bio-Oil to Alkanes†

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Highly Selective Catalytic Conversion of Phenolic Bio-Oil to Alkanes^†