Spontaneous Formation of Ordered 3D Superlattices of Nanocrystals from Polydisperse Colloidal Solutions†
Katerina Soulantica Dr.
Laboratoire de Chimie de Coordination du CNRS, 205, route de Narbonne, 31077 Toulouse, France, Fax: (+33) 5-6155-3003
Search for more papers by this authorAndré Maisonnat Dr.
Laboratoire de Chimie de Coordination du CNRS, 205, route de Narbonne, 31077 Toulouse, France, Fax: (+33) 5-6155-3003
Search for more papers by this authorMarie-Claire Fromen
Centre d'Elaboration des Matériaux et, d'Etudes Structurales du CNRS, 29, rue Jeanne Marvig BP 4347, 31055 Toulouse, France
Search for more papers by this authorMarie-José Casanove Dr.
Centre d'Elaboration des Matériaux et, d'Etudes Structurales du CNRS, 29, rue Jeanne Marvig BP 4347, 31055 Toulouse, France
Search for more papers by this authorBruno Chaudret Dr.
Laboratoire de Chimie de Coordination du CNRS, 205, route de Narbonne, 31077 Toulouse, France, Fax: (+33) 5-6155-3003
Search for more papers by this authorKaterina Soulantica Dr.
Laboratoire de Chimie de Coordination du CNRS, 205, route de Narbonne, 31077 Toulouse, France, Fax: (+33) 5-6155-3003
Search for more papers by this authorAndré Maisonnat Dr.
Laboratoire de Chimie de Coordination du CNRS, 205, route de Narbonne, 31077 Toulouse, France, Fax: (+33) 5-6155-3003
Search for more papers by this authorMarie-Claire Fromen
Centre d'Elaboration des Matériaux et, d'Etudes Structurales du CNRS, 29, rue Jeanne Marvig BP 4347, 31055 Toulouse, France
Search for more papers by this authorMarie-José Casanove Dr.
Centre d'Elaboration des Matériaux et, d'Etudes Structurales du CNRS, 29, rue Jeanne Marvig BP 4347, 31055 Toulouse, France
Search for more papers by this authorBruno Chaudret Dr.
Laboratoire de Chimie de Coordination du CNRS, 205, route de Narbonne, 31077 Toulouse, France, Fax: (+33) 5-6155-3003
Search for more papers by this authorThe authors thank the CNRS and EC (through TMR netwok CLUPOS) for support. We express our gratitude to Professors. Pablo Espinet and John Bradley for fruitful discussions, Dr. F. Senocq for XRD measurements, and M. Vincent Collière, Lucien Datas, and the TEMSCAN service for TEM studies.
Graphical Abstract
Ordnung durch Fluktuation: Aus einer nichtgeordneten Dispersion kristallisieren spontan hoch geordnete Nanokristall-Übergitter von identischen Zinnpartikeln. Zwei Strukturtypen wurden identifiziert: ein nichtkompakter mit einheitlich orientierten Atomebenen der Partikel und einer mit monodispersen und stärker anisotrop geordneten Partikeln (siehe elektronenmikrokopische Aufnahmen). Welche Struktur gebildet wird, hängt von den Reaktionsbedingungen ab.
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