Model-Based Optimization of a Photocatalytic Reactor with Light-Emitting Diodes
Fatemeh Khodadadian
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorAli Poursaeidesfahani
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorZonghan Li
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorJ. Ruud van Ommen
Chemical Engineering Department, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorAndrzej I. Stankiewicz
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorCorresponding Author
Richard Lakerveld
Department of Chemical and Biomolecular Engineering, The Hong Kong Universityof Science and Technology, Hong Kong.
Department of Chemical and Biomolecular Engineering, The Hong Kong Universityof Science and Technology, Hong Kong.Search for more papers by this authorFatemeh Khodadadian
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorAli Poursaeidesfahani
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorZonghan Li
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorJ. Ruud van Ommen
Chemical Engineering Department, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorAndrzej I. Stankiewicz
Department of Process & Energy, Delft University of Technology, Delft, The Netherlands.
Search for more papers by this authorCorresponding Author
Richard Lakerveld
Department of Chemical and Biomolecular Engineering, The Hong Kong Universityof Science and Technology, Hong Kong.
Department of Chemical and Biomolecular Engineering, The Hong Kong Universityof Science and Technology, Hong Kong.Search for more papers by this authorAbstract
The complicated interplay between mass and photon transfer within a photocatalytic reactor calls for an integrated design approach. A model-based optimization approach for LED-based photocatalytic reactors is presented. First, a model that describes the distribution of reactants and photons within a photocatalytic reactor is developed. Then, several design variables related to the reactor dimensions and light sources are optimized simultaneously using the photocatalytic degradation of toluene as a model system. The results demonstrate how different formulations of the problem can be used to either minimize the reactor cost or to obtain a specified concentration profile within the reactor.
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