Eco-friendly and facile modified superhydrophobic melamine sponge by molybdenum sulfide for oil/water separation
Lei Li
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Data curation (equal), Methodology (equal), Validation (equal), Writing - original draft (equal), Writing - review & editing (equal)
Search for more papers by this authorRui Chen
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Methodology (equal), Writing - review & editing (equal)
Search for more papers by this authorFengyu Wen
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Investigation (equal), Writing - review & editing (equal)
Search for more papers by this authorYashu He
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Investigation (equal), Methodology (equal)
Search for more papers by this authorLin Cheng
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Data curation (equal), Software (equal)
Search for more papers by this authorJierun Ma
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Data curation (equal), Software (equal)
Search for more papers by this authorCorresponding Author
Jianxin Mu
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Correspondence
Jianxin Mu, Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun 130012, People's Republic of China.
Email: [email protected]
Contribution: Project administration (equal), Supervision (equal), Writing - review & editing (equal)
Search for more papers by this authorLei Li
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Data curation (equal), Methodology (equal), Validation (equal), Writing - original draft (equal), Writing - review & editing (equal)
Search for more papers by this authorRui Chen
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Methodology (equal), Writing - review & editing (equal)
Search for more papers by this authorFengyu Wen
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Investigation (equal), Writing - review & editing (equal)
Search for more papers by this authorYashu He
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Investigation (equal), Methodology (equal)
Search for more papers by this authorLin Cheng
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Data curation (equal), Software (equal)
Search for more papers by this authorJierun Ma
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Contribution: Data curation (equal), Software (equal)
Search for more papers by this authorCorresponding Author
Jianxin Mu
Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun, People's Republic of China
Correspondence
Jianxin Mu, Key Laboratory of High Performance Plastics, Ministry of Education, National & Local Joint Engineering Laboratory for Synthesis Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun 130012, People's Republic of China.
Email: [email protected]
Contribution: Project administration (equal), Supervision (equal), Writing - review & editing (equal)
Search for more papers by this authorAbstract
Oily wastewater has caused serious damage to the human health and ecological environment. It is urgent to develop novel materials for high performance oil/water separation. Porous melamine sponges (MS) are considered as an ideal matrix material for oil/water separation. Herein, molybdenum sulfide (MoS2) modified with tannic acid (TA) and octadecylamine (ODA) was attached to MS framework via a facile dip-coating method. This novel and eco-friendly MS@(MoS2@ODA) sponge displays superior superhydrophobicity (WCA = 156.2°) and oil/water separation ability (absorption capacity = 113–145 g g−1). MoS2@ODA not only enhances surface roughness of MS framework, but also raises its specific surface area, causing an increase in the oil adsorption capacity of MS. Moreover, the composite sponge exhibited excellent chemical and mechanical stability. It is envisioned that this work can demonstrate a facile synthesis strategy for producing environmental friendliness MS with stable superhydrophobicity for high-efficient oil/water separation.
CONFLICT OF INTEREST STATEMENT
The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
Open Research
DATA AVAILABILITY STATEMENT
The data that support the findings of this study are available from the corresponding author upon seasonable request.
Supporting Information
| Filename | Description |
|---|---|
| app53875-sup-0001-Supinfo.docxWord 2007 document , 239.3 KB | Figure S1 FTIR (a) and XPS (b) spectrum of TA and ODA, the C1s (c) and O1s (d) spectrum of TA. |
| app53875-sup-0002-MovieS1.mp4MPEG-4 video, 1.7 MB | Movie S1 Surface wetting behavior of pristine MS. |
| app53875-sup-0003-MovieS2.mp4MPEG-4 video, 8.7 MB | Movie S2 Surface wetting behavior of modified MS. |
| app53875-sup-0004-MovieS3.mp4MPEG-4 video, 13.5 MB | Movie S3 Light oil adsorption on water surface. |
| app53875-sup-0005-MovieS4.mp4MPEG-4 video, 6.2 MB | Movie S4 Heavy oil adsorption under water. |
Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.
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