Aluminoborates as Nonlinear Optical Materials
Jiahao Jiao
Research Center for Crystal Materials, CAS Key Laboratory of Functional Materials and Devices for Special Environments, Xinjiang Technical Institute of Physics & Chemistry, CAS, 40-1 South Beijing Road, Urumqi, 830011 China
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049 China
Search for more papers by this authorCorresponding Author
Prof. Min Zhang
Research Center for Crystal Materials, CAS Key Laboratory of Functional Materials and Devices for Special Environments, Xinjiang Technical Institute of Physics & Chemistry, CAS, 40-1 South Beijing Road, Urumqi, 830011 China
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049 China
Search for more papers by this authorCorresponding Author
Prof. Shilie Pan
Research Center for Crystal Materials, CAS Key Laboratory of Functional Materials and Devices for Special Environments, Xinjiang Technical Institute of Physics & Chemistry, CAS, 40-1 South Beijing Road, Urumqi, 830011 China
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049 China
Search for more papers by this authorJiahao Jiao
Research Center for Crystal Materials, CAS Key Laboratory of Functional Materials and Devices for Special Environments, Xinjiang Technical Institute of Physics & Chemistry, CAS, 40-1 South Beijing Road, Urumqi, 830011 China
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049 China
Search for more papers by this authorCorresponding Author
Prof. Min Zhang
Research Center for Crystal Materials, CAS Key Laboratory of Functional Materials and Devices for Special Environments, Xinjiang Technical Institute of Physics & Chemistry, CAS, 40-1 South Beijing Road, Urumqi, 830011 China
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049 China
Search for more papers by this authorCorresponding Author
Prof. Shilie Pan
Research Center for Crystal Materials, CAS Key Laboratory of Functional Materials and Devices for Special Environments, Xinjiang Technical Institute of Physics & Chemistry, CAS, 40-1 South Beijing Road, Urumqi, 830011 China
Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049 China
Search for more papers by this authorAbstract
Ultraviolet (UV) and Deep-UV (DUV, λ<200 nm) nonlinear optical (NLO) materials play a significant role to convert the wavelength of laser for producing UV/DUV coherent light in the laser industry. The Al [Ne]3s23p1 atom with empty d orbitals can form sp3, sp3d, and sp3d2 hybrid orbitals when bonding with O/F atoms, which leads to the construction of [AlOmFn] (m+n=4, 5, 6) units. Therein, aluminoborates have received intensive attention due to the effective structural and functional adjustment effects of the diverse Al−O/F units. Accordingly, numerous aluminoborates as candidates for the next generation of UV/DUV NLO materials were discovered. In this review, recently discovered aluminoborates are overviewed and analyzed, including their syntheses, crystal structure features, and second-order NLO performances. We aim to provide the latest progress and outlook on the crystal chemistry of aluminoborates and boost the finding of the next NLO candidates with high performances.
Conflict of interest
The authors declare no conflict of interest.
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