Terminal Group-Oriented Self-Assembly to Controllably Synthesize a Layer-by-Layer SnSe2 and MXene Heterostructure for Ultrastable Lithium Storage
Xianglong Kong
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorXiaohan Zhao
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorChen Li
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorZhuoming Jia
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorCorresponding Author
Chengkai Yang
College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108 P. R. China
E-mail: [email protected]; [email protected]; [email protected]
Search for more papers by this authorZhuoyan Wu
Comprehensive Energy Research Center, Institute of Science and Technology, China Three Gorges Corporation, Beijing, 100038 P. R. China
Search for more papers by this authorXudong Zhao
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorYing Zhao
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorFei He
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorYueming Ren
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorCorresponding Author
Piaoping Yang
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
E-mail: [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Zhiliang Liu
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
E-mail: [email protected]; [email protected]; [email protected]
Search for more papers by this authorXianglong Kong
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorXiaohan Zhao
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorChen Li
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorZhuoming Jia
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorCorresponding Author
Chengkai Yang
College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108 P. R. China
E-mail: [email protected]; [email protected]; [email protected]
Search for more papers by this authorZhuoyan Wu
Comprehensive Energy Research Center, Institute of Science and Technology, China Three Gorges Corporation, Beijing, 100038 P. R. China
Search for more papers by this authorXudong Zhao
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorYing Zhao
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorFei He
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorYueming Ren
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
Search for more papers by this authorCorresponding Author
Piaoping Yang
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
E-mail: [email protected]; [email protected]; [email protected]
Search for more papers by this authorCorresponding Author
Zhiliang Liu
College of Material Sciences and Chemical Engineering, Harbin Engineering University, Harbin, 150001 P. R. China
E-mail: [email protected]; [email protected]; [email protected]
Search for more papers by this authorAbstract
Heterostructured materials integrate the advantages of adjustable electronic structure, fast electron/ions transfer kinetics, and robust architectures, which have attracted considerable interest in the fields of rechargeable batteries, photo/electrocatalysis, and supercapacitors. However, the construction of heterostructures still faces some severe problems, such as inferior random packing of components and serious agglomeration. Herein, a terminal group-oriented self-assembly strategy to controllably synthesize a homogeneous layer-by-layer SnSe2 and MXene heterostructure (LBL-SnSe2@MXene) is designed. Benefitting from the abundant polar terminal groups on the MXene surface, Sn2+ is induced into the interlayer of MXene with large interlayer spacing, which is selenized in situ to obtain LBL-SnSe2@MXene. In the heterostructure, SnSe2 layers and MXene layers are uniformly intercalated in each other, superior to other heterostructures formed by random stacking. As an anode for lithium-ion batteries, the LBL-SnSe2@MXene is revealed to possess strong lithium adsorption ability, the small activation energy for lithium diffusion, and excellent structure stability, thus achieving outstanding electrochemical performance, especially with high specific capacities (1311 and 839 mAh g−1 for initial discharge and charge respectively) and ultralong cycling stability (410 mAh g−1 at 5C even after 16 000 cycles). This work conveys an inspiration for the controllable design and construction of homogeneous layered heterostructures.
Conflict of Interest
The authors declare no conflict of interest.
Open Research
Data Availability Statement
The data that support the findings of this study are available from the corresponding author upon reasonable request.
Supporting Information
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