Absorption of CO2 with Amino Acid-Based Ionic Liquids and Corresponding Amino Acid Precursors
Javier Guzmán
Instituto Mexicano del Petróleo, Gerencia de Refinación de Hidrocarburos, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Search for more papers by this authorChristian Ortega-Guevara
Instituto Mexicano del Petróleo, Gerencia de Refinación de Hidrocarburos, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Search for more papers by this authorRoberto García de León
Instituto Mexicano del Petróleo, Gerencia de Refinación de Hidrocarburos, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Search for more papers by this authorCorresponding Author
Rafael Martínez-Palou
Instituto Mexicano del Petróleo, Gerencia de Transformación de Biomasa, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Correspondence: Rafael Martínez-Palou ([email protected]), Instituto Mexicano del Petróleo, Gerencia de Transformación de Biomasa, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico.Search for more papers by this authorJavier Guzmán
Instituto Mexicano del Petróleo, Gerencia de Refinación de Hidrocarburos, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Search for more papers by this authorChristian Ortega-Guevara
Instituto Mexicano del Petróleo, Gerencia de Refinación de Hidrocarburos, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Search for more papers by this authorRoberto García de León
Instituto Mexicano del Petróleo, Gerencia de Refinación de Hidrocarburos, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Search for more papers by this authorCorresponding Author
Rafael Martínez-Palou
Instituto Mexicano del Petróleo, Gerencia de Transformación de Biomasa, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico
Correspondence: Rafael Martínez-Palou ([email protected]), Instituto Mexicano del Petróleo, Gerencia de Transformación de Biomasa, Eje Central Lázaro Cárdenas 152, 07730 Mexico City, Mexico.Search for more papers by this authorAbstract
A comparative study for CO2 absorption among amino acids (AAs) and ionic liquids (ILs) containing tetramethylammonium [TMA] and tetrabutylphosphonium [TBP] as cations and the corresponding deprotonated amino acid as anions, namely, [TMA][AA] and [TBP][AA], is reported. Amino acids show an excellent performance for CO2 capture, better than the corresponding [TMA][AA], but AAs are less efficient than [TBP][AA]. In addition, [TBP][AA] present faster kinetics of absorption than the corresponding AA. [TBP][lysinate] exhibits the highest CO2 absorption capacity. A novel and fast method with low energy demand for microwave-assisted regeneration of the absorbents from the CO2-saturated solution is also described for the first time.
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