Volume 136, Issue 33 e202412574

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Rücktitelbild: Light-Induced Dynamic Activation of Copper/Silicon Interface for Highly Selective Carbon Dioxide Reduction (Angew. Chem. 33/2024)

Jiali Wang

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

These authors contributed equally.

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Tai Ying Lai,

Tai Ying Lai

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

These authors contributed equally.

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Han-Ting Lin,

Han-Ting Lin

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

These authors contributed equally.

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Tsung-Rong Kuo,

Corresponding Author

Tsung-Rong Kuo

[email protected]

Graduate Institute of Nanomedicine and Medical Engineering, College of Biomedical Engineering, Taipei Medical University, Taipei, 11031 Taiwan

Precision Medicine and Translational Cancer Research Center, Taipei Medical University Hospital, Taipei, 11031 Taiwan

These authors contributed equally.

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Hsiao-Chien Chen,

Hsiao-Chien Chen

orcid.org/0000-0002-7480-9940

Center for Reliability Sciences and Technologies, Chang Gung University, Taoyuan, 333 Taiwan

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Chun-Sheng Tseng,

Chun-Sheng Tseng

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

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Ching-Wei Tung,

Corresponding Author

Ching-Wei Tung

[email protected]

Center for Environmental Sustainability and Human Health, Ming Chi University of Technology, New Taipei City, 24301 Taiwan

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Chia-Ying Chien,

Chia-Ying Chien

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

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Hao Ming Chen,

Corresponding Author

Hao Ming Chen

[email protected]

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

National Synchrotron Radiation Research Center, Hsinchu, 30076 Taiwan

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Jiali Wang,

Jiali Wang

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

These authors contributed equally.

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Tai Ying Lai,

Tai Ying Lai

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

These authors contributed equally.

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Han-Ting Lin,

Han-Ting Lin

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

These authors contributed equally.

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Tsung-Rong Kuo,

Corresponding Author

Tsung-Rong Kuo

[email protected]

Graduate Institute of Nanomedicine and Medical Engineering, College of Biomedical Engineering, Taipei Medical University, Taipei, 11031 Taiwan

Precision Medicine and Translational Cancer Research Center, Taipei Medical University Hospital, Taipei, 11031 Taiwan

These authors contributed equally.

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Hsiao-Chien Chen,

Hsiao-Chien Chen

orcid.org/0000-0002-7480-9940

Center for Reliability Sciences and Technologies, Chang Gung University, Taoyuan, 333 Taiwan

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Chun-Sheng Tseng,

Chun-Sheng Tseng

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

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Ching-Wei Tung,

Corresponding Author

Ching-Wei Tung

[email protected]

Center for Environmental Sustainability and Human Health, Ming Chi University of Technology, New Taipei City, 24301 Taiwan

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Chia-Ying Chien,

Chia-Ying Chien

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

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Hao Ming Chen,

Corresponding Author

Hao Ming Chen

[email protected]

Department of Chemistry and Center for Emerging Materials and Advanced Devices, National Taiwan University, Taipei, 10617 Taiwan

National Synchrotron Radiation Research Center, Hsinchu, 30076 Taiwan

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First published: 11 July 2024

https://doi.org/10.1002/ange.202412574

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Graphical Abstract

Light-induced dynamic metal nanocrystal/semiconductor interfaces during carbon dioxide electroreduction were investigated by utilizing synchrotron radiation X-ray absorption spectroscopy, as reported by Hao Ming Chen et al. in their Research Article (e202403333). The dynamic structural transformations of metal/semiconductor junction under illumination result in an intriguing selectivity switch and realize an improvement of at least 16-fold in the product ratio of CH₄/C₂ products.