Review
Porphyrin-Based Metal-Organic Framework Photocatalysts: Structure, Mechanism and Applications
Xiansheng Zhang,
Zhifeng Liu,
Binbin Shao,
Qinghua Liang,
Ting Wu,
Yuan Pan,
Qingyun He,
Miao He,
Lin Ge,
Jian Huang,
Xiansheng Zhang
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorCorresponding Author
Zhifeng Liu
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
E-mail: [email protected]
Search for more papers by this authorBinbin Shao
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorQinghua Liang
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorTing Wu
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorYuan Pan
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorQingyun He
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorMiao He
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorLin Ge
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorJian Huang
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorXiansheng Zhang,
Zhifeng Liu,
Binbin Shao,
Qinghua Liang,
Ting Wu,
Yuan Pan,
Qingyun He,
Miao He,
Lin Ge,
Jian Huang,
Xiansheng Zhang
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorCorresponding Author
Zhifeng Liu
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
E-mail: [email protected]
Search for more papers by this authorBinbin Shao
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorQinghua Liang
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorTing Wu
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorYuan Pan
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorQingyun He
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorMiao He
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorLin Ge
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorJian Huang
College of Environmental Science and Engineering, Hunan University and Key Laboratory of Environmental Biology and Pollution Control (Hunan University), Ministry of Education, Changsha, 410082 P. R. China
Search for more papers by this authorAbstract
In recent years, porphyrins have been frequently reported as photocatalysts due to their fascinating photochemical properties. However, porphyrins have the same shortcomings as other homogeneous photocatalysts, such as poor stability and difficulty in recovering. To solve this problem, it is a good strategy to form a porphyrin-based metal-organic framework (PMOF) by modifying porphyrin functional groups and adding metals as nodes to connect and control the arrangement of porphyrins. The metal nodes control the rigidity and connectivity of the porphyrin modules to order them in the MOF, which improves the stability of the porphyrins, avoids porphyrin aggregation and folding, and increases the active sites for photocatalytic reactions. This review summarized the research progress of PMOF photocatalysts in the last ten years and analyzed the effects of the spatial structure, porphyrin ligands, porphyrin central metals, and metal nodes of PMOF on the photocatalytic performance. The applications of PMOF-based photocatalysts in H2 production, CO2 reduction, pollutant degradation, and sterilization are reviewed. In addition, the mechanism of these processes is described in detail. Finally, some suggestions on the development of PMOF photocatalysts are put forward.
Conflict of Interest
The authors declare no conflict of interest.
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