Facilitating CO2–CH4 Reforming Into Syngas and Useful Chemicals by Water-Cooled Dielectric Barrier Discharge Plasma: Effect of Discharge Power, Gas Mixing, and Mechanism Insight
Corresponding Author
Tian Chang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an, China
State Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering, Ningxia University, Yinchuan, China
Correspondence: Tian Chang ([email protected])
Search for more papers by this authorXuanchen Chang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorAbdelkader Labidi
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorChuanlong Ma
Research Unit Plasma Technology (RUPT), Department of Applied Physics, Faculty of Engineering and Architecture, Ghent University, Ghent, Belgium
Search for more papers by this authorZuotong Zhao
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorZerong Jiang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorZhao Yang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorYuqin Wang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorChuanyi Wang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorCorresponding Author
Tian Chang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an, China
State Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering, Ningxia University, Yinchuan, China
Correspondence: Tian Chang ([email protected])
Search for more papers by this authorXuanchen Chang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorAbdelkader Labidi
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorChuanlong Ma
Research Unit Plasma Technology (RUPT), Department of Applied Physics, Faculty of Engineering and Architecture, Ghent University, Ghent, Belgium
Search for more papers by this authorZuotong Zhao
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorZerong Jiang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorZhao Yang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorYuqin Wang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorChuanyi Wang
School of Environmental Science and Engineering, Shaanxi University of Science and Technology, Xi'an, China
Search for more papers by this authorABSTRACT
CO2 reforming of CH4 to syngas (H2 and CO) has emerged as one of the attractive options for mitigating carbon emissions. Here, a water-cooled dielectric barrier discharge plasma reactor has been constructed for CO2–CH4 reforming to produce syngas and value-added chemicals. The effects of the main parameters (i.e., discharge power, CH4/CO2 molar ratio, and gas flow rate) on CO2–CH4 reforming were investigated. The highest conversion rate of CH4 and CO2 was found to be 40.57% and 27.15%, respectively, with CO and H2 selectivity of 56.07% and 43.71%, respectively. The total energy efficiency achieved was 0.28 mmol/kJ. C2H6 was found to be the main hydrocarbon product. Lastly, the mechanism of CO2–CH4 reforming was proposed in terms of the active species and products.
Conflicts of Interest
The authors declare no conflicts of interest.
Open Research
Data Availability Statement
The authors have nothing to report.
Supporting Information
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