Ionic Liquids and their Polymers in Lithium-Sulfur Batteries
Elinor Josef
Max Planck Institute of Colloids and Interfaces, Department of Colloid Chemistry, Am Mühlenberg 1, 14476 Potsdam, Germany
Search for more papers by this authorYajing Yan
Department of Physics, Chalmers University of Technology, SE-41296 Göteborg, Sweden
Search for more papers by this authorMarian Cristian Stan
MEET Battery Research Center, University of Münster, Corrennstrasse 46, 48149 Münster, Germany
Search for more papers by this authorJulia Wellmann
MEET Battery Research Center, University of Münster, Corrennstrasse 46, 48149 Münster, Germany
Search for more papers by this authorAlen Vizintin
National Institute of Chemistry, Hajdrihova 19, 1000 Ljubljana, Slovenia, Faculty of Chemistry and Chemical Technology, University of Ljubljana, Večna pot 113, 1000 Ljubljana, Slovenia
Search for more papers by this authorMartin Winter
MEET Battery Research Center, University of Münster, Corrennstrasse 46, 48149 Münster, Germany
Helmholz-Institute Münster (HI MS), IEK-12 of Forschungszentrum Jülich, Corrensstrasse 46, 48149 Münster, Germany
Search for more papers by this authorPatrik Johansson
Department of Physics, Chalmers University of Technology, SE-41296 Göteborg, Sweden
ALISTORE-European Research Institute, CNRS FR 3104, Hub de l'Energie, Rue Baudelocque, 80039 Amiens, France
Search for more papers by this authorRobert Dominko
National Institute of Chemistry, Hajdrihova 19, 1000 Ljubljana, Slovenia, Faculty of Chemistry and Chemical Technology, University of Ljubljana, Večna pot 113, 1000 Ljubljana, Slovenia
ALISTORE-European Research Institute, CNRS FR 3104, Hub de l'Energie, Rue Baudelocque, 80039 Amiens, France
Search for more papers by this authorCorresponding Author
Ryan Guterman
Max Planck Institute of Colloids and Interfaces, Department of Colloid Chemistry, Am Mühlenberg 1, 14476 Potsdam, Germany
Search for more papers by this authorElinor Josef
Max Planck Institute of Colloids and Interfaces, Department of Colloid Chemistry, Am Mühlenberg 1, 14476 Potsdam, Germany
Search for more papers by this authorYajing Yan
Department of Physics, Chalmers University of Technology, SE-41296 Göteborg, Sweden
Search for more papers by this authorMarian Cristian Stan
MEET Battery Research Center, University of Münster, Corrennstrasse 46, 48149 Münster, Germany
Search for more papers by this authorJulia Wellmann
MEET Battery Research Center, University of Münster, Corrennstrasse 46, 48149 Münster, Germany
Search for more papers by this authorAlen Vizintin
National Institute of Chemistry, Hajdrihova 19, 1000 Ljubljana, Slovenia, Faculty of Chemistry and Chemical Technology, University of Ljubljana, Večna pot 113, 1000 Ljubljana, Slovenia
Search for more papers by this authorMartin Winter
MEET Battery Research Center, University of Münster, Corrennstrasse 46, 48149 Münster, Germany
Helmholz-Institute Münster (HI MS), IEK-12 of Forschungszentrum Jülich, Corrensstrasse 46, 48149 Münster, Germany
Search for more papers by this authorPatrik Johansson
Department of Physics, Chalmers University of Technology, SE-41296 Göteborg, Sweden
ALISTORE-European Research Institute, CNRS FR 3104, Hub de l'Energie, Rue Baudelocque, 80039 Amiens, France
Search for more papers by this authorRobert Dominko
National Institute of Chemistry, Hajdrihova 19, 1000 Ljubljana, Slovenia, Faculty of Chemistry and Chemical Technology, University of Ljubljana, Večna pot 113, 1000 Ljubljana, Slovenia
ALISTORE-European Research Institute, CNRS FR 3104, Hub de l'Energie, Rue Baudelocque, 80039 Amiens, France
Search for more papers by this authorCorresponding Author
Ryan Guterman
Max Planck Institute of Colloids and Interfaces, Department of Colloid Chemistry, Am Mühlenberg 1, 14476 Potsdam, Germany
Search for more papers by this authorGraphical Abstract
Abstract
Future optimized lithium-sulfur batteries may promise higher energy densities than the current standard. However, there are many barriers which hinder their commercialization. In this review we describe how ionic liquids (ILs) and their polymers are utilized in different components of the battery to address some of these issues. For example, IL-based electrolytes have the potential to reduce the solubility of polysulfides compared to conventional organic electrolytes. Polymerizing ILs directly on the surface of the Li-metal anode is suggested as an approach to protect the surface of this electrode. Finally, using poly(ionic liquids) (PILs) as binders for the cathode active material may increase the performance of the cathode as compared to polyvinylidene difluoride (PVdF) and could inhibit swelling-induced degradation. These results demonstrate the advantages of ILs and their polymers for improving the performance of Li−S batteries.
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