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Single-molecule magnets (SMMs) are widely recognized as promising candidates for high-density storage and quantum processing of information. The relationship between property and structure is fundamental in the design of high-performance SMMs. A detailed study of the relaxation dynamics and structures in two sandwich-type Er(III) SMMs with ansa-cyclooctatetraenyl ligands has highlighted the positive contribution of dipolar interactions to the magnetic blocking of SMMs. More details are discussed in the article by Ding et al. on pages 3099—3106.