Acidification Optimization and Granulation of a Steel-Slag-Derived Sorbent for CO2 Capture
Jian Sun
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Nanjing Normal University, Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, 78 Bancang Street, 210042 Nanjing, China
Search for more papers by this authorCorresponding Author
Wenqiang Liu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Correspondence: Wenqiang Liu ([email protected]), Minghou Xu ([email protected]), State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan 430074, China.Search for more papers by this authorYingchao Hu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Search for more papers by this authorYuandong Yang
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Search for more papers by this authorYongqing Xu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Search for more papers by this authorCorresponding Author
Minghou Xu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Correspondence: Wenqiang Liu ([email protected]), Minghou Xu ([email protected]), State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan 430074, China.Search for more papers by this authorJian Sun
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Nanjing Normal University, Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, 78 Bancang Street, 210042 Nanjing, China
Search for more papers by this authorCorresponding Author
Wenqiang Liu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Correspondence: Wenqiang Liu ([email protected]), Minghou Xu ([email protected]), State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan 430074, China.Search for more papers by this authorYingchao Hu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Search for more papers by this authorYuandong Yang
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Search for more papers by this authorYongqing Xu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Search for more papers by this authorCorresponding Author
Minghou Xu
Huazhong University of Science and Technology, State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, 1037 Luoyu Road, 430074 Wuhan, China
Correspondence: Wenqiang Liu ([email protected]), Minghou Xu ([email protected]), State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, 1037 Luoyu Road, Wuhan 430074, China.Search for more papers by this authorAbstract
Steel slag was used as a low-cost feedstock to prepare CaO-based sorbents for CO2 capture by acidification treatment, and the acidification process was optimized. Four main acidification parameters (i.e., extraction time, extraction temperature, acetic acid concentration, and solid/liquid ratio) were investigated. The solid/liquid ratio and extraction time are the most important factors that affect the CO2 capture capacity and stability of the sorbents. The CO2 sorption performance of optimal steel-slag-derived sorbent is more stable than that of naturally occurring limestone, due to the low Si/Ca ratio and the presence of MgO with high anti-sintering ability. CaO-based pellets with high resistance to attrition and compression were produced by extrusion of the steel-slag-derived sorbent powders.
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