Review
Progress on Lithium Dendrite Suppression Strategies from the Interior to Exterior by Hierarchical Structure Designs
Lu Shen,
Peiran Shi,
Xiaoge Hao,
Qiang Zhao,
Jiabin Ma,
Yan-Bing He,
Feiyu Kang,
Lu Shen
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorPeiran Shi
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorXiaoge Hao
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorQiang Zhao
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorJiabin Ma
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorCorresponding Author
Yan-Bing He
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
E-mail: [email protected], [email protected]
Search for more papers by this authorCorresponding Author
Feiyu Kang
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
E-mail: [email protected], [email protected]
Search for more papers by this authorLu Shen,
Peiran Shi,
Xiaoge Hao,
Qiang Zhao,
Jiabin Ma,
Yan-Bing He,
Feiyu Kang,
Lu Shen
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorPeiran Shi
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorXiaoge Hao
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorQiang Zhao
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorJiabin Ma
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
Search for more papers by this authorCorresponding Author
Yan-Bing He
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
E-mail: [email protected], [email protected]
Search for more papers by this authorCorresponding Author
Feiyu Kang
Shenzhen Geim Graphene, Center Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen, 518055 P. R. China
Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua University, Beijing, 100084 P. R. China
E-mail: [email protected], [email protected]
Search for more papers by this authorAbstract
Lithium (Li) metal is promising for high energy density batteries due to its low electrochemical potential (−3.04 V) and high specific capacity (3860 mAh g−1). However, the safety issues impede the commercialization of Li anode batteries. In this work, research of hierarchical structure designs for Li anodes to suppress Li dendrite growth and alleviate volume expansion from the interior (by the 3D current collector and host matrix) to the exterior (by the artificial solid electrolyte interphase (SEI), protective layer, separator, and solid state electrolyte) is concluded. The basic principles for achieving Li dendrite and volume expansion free Li anode are summarized. Following these principles, 3D porous current collector and host matrix are designed to suppress the Li dendrite growth from the interior. Second, artificial SEI, the protective layer, and separator as well as solid-state electrolyte are constructed to regulate the distribution of current and control the Li nucleation and deposition homogeneously for suppressing the Li dendrite growth from exterior of Li anode. Ultimately, this work puts forward that it is significant to combine the Li dendrite suppression strategies from the interior to exterior by 3D hierarchical structure designs and Li metal modification to achieve excellent cycling and safety performance of Li metal batteries.
Conflict of Interest
The authors declare no conflict of interest.
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