Volume 45, Issue 14 2400105

Research Article

Shape Memory Polyurethane Composite With Fast Response to Near-Infrared Light Based on Tannic Acid–Iron and Dynamic Phenol-Carbamate Network

Yong Yong,

Yong Yong

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Yang Liu,

Yang Liu

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Zetian Zhang,

Zetian Zhang

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Songbo Dai,

Songbo Dai

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Xiaohan Yang,

Xiaohan Yang

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Fufen Li,

Fufen Li

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Zhengjun Li,

Corresponding Author

Zhengjun Li

[email protected]

orcid.org/0000-0002-3943-5621

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

: [email protected]

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Yong Yong,

Yong Yong

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Yang Liu,

Yang Liu

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Zetian Zhang,

Zetian Zhang

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Songbo Dai,

Songbo Dai

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Xiaohan Yang,

Xiaohan Yang

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Fufen Li,

Fufen Li

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

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Zhengjun Li,

Corresponding Author

Zhengjun Li

[email protected]

orcid.org/0000-0002-3943-5621

College of Biomass Science and Engineering, Sichuan University, Chengdu, 610065 China

Key Laboratory of Leather Chemistry and Engineering of Ministry of Education, Sichuan University, Chengdu, 610065 China

: [email protected]

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First published: 16 April 2024

https://doi.org/10.1002/marc.202400105

Citations: 2

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Abstract

Intelligent materials derived from green and renewable bio-based materials garner widespread attention recently. Herein, shape memory polyurethane composite (PUTA/Fe) with fast response to near-infrared (NIR) light is successfully prepared by introducing Fe³⁺ into the tannic acid-based polyurethane (PUTA) matrix through coordination between Fe³⁺ and tannic acid. The results show that the excellent NIR light response ability is due to the even distribution of Fe³⁺ filler with good photo-thermal conversion ability. With the increase of Fe³⁺ content, the NIR light response shape recovery rate of PUTA/Fe composite films is significantly improved, and the shape recovery time is reduced from over 60 s to 40 s. In addition, the mechanical properties of PUTA/Fe composite film are also improved. Importantly, owing to the dynamic phenol–carbamate network within the polymer matrix, the PUTA/Fe composite film can reshape its permanent shape through topological rearrangement and show its good NIR light response shape memory performance. Therefore, PUTA/Fe composites with high content of bio-based material (TA content of 15.1–19.4%) demonstrate the shape memory characteristics of fast response to NIR light; so, it will have great potential in the application of new intelligent materials including efficient and environmentally friendly smart photothermal responder.

Conflict of Interest

The authors declare no conflict of interest.

Open Research

Data Availability Statement

The data that support the findings of this study are available from the corresponding author upon reasonable request.

Supporting Information

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Volume45, Issue14

July 2024

2400105

Filename	Description
marc202400105-sup-0001-SuppMat.docx246.4 KB	Supporting Information
marc202400105-sup-0002-MovieS1.mp45.3 MB	Supplemental Movie 1
marc202400105-sup-0003-MovieS2.mp44.6 MB	Supplemental Movie 2

Shape Memory Polyurethane Composite With Fast Response to Near-Infrared Light Based on Tannic Acid–Iron and Dynamic Phenol-Carbamate Network

Abstract

Conflict of Interest

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Data Availability Statement

Supporting Information

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Shape Memory Polyurethane Composite With Fast Response to Near-Infrared Light Based on Tannic Acid–Iron and Dynamic Phenol-Carbamate Network

Abstract

Conflict of Interest

Open Research

Data Availability Statement

Supporting Information

References

Citing Literature

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